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Fusion Science and Technology
Latest News
Glass strategy: Hanford’s enhanced waste glass program
The mission of the Department of Energy’s Office of River Protection (ORP) is to complete the safe cleanup of waste resulting from decades of nuclear weapons development. One of the most technologically challenging responsibilities is the safe disposition of approximately 56 million gallons of radioactive waste historically stored in 177 tanks at the Hanford Site in Washington state.
ORP has a clear incentive to reduce the overall mission duration and cost. One pathway is to develop and deploy innovative technical solutions that can advance baseline flow sheets toward higher efficiency operations while reducing identified risks without compromising safety. Vitrification is the baseline process that will convert both high-level and low-level radioactive waste at Hanford into a stable glass waste form for long-term storage and disposal.
Although vitrification is a mature technology, there are key areas where technology can further reduce operational risks, advance baseline processes to maximize waste throughput, and provide the underpinning to enhance operational flexibility; all steps in reducing mission duration and cost.
H. Kakiuchi et al.
Fusion Science and Technology | Volume 60 | Number 4 | November 2011 | Pages 1256-1259
Environmental and Organically Bound Tritium | Proceedings of the Ninth International Conference on Tritium Science and Technology (Part 2) | doi.org/10.13182/FST11-A12658
Articles are hosted by Taylor and Francis Online.
We developed an analytical method for organically bound 3H (OBT) in biological environmental samples by using noble gas mass spectrometry of 3He produced from 3H. Three environmental samples with background level OBT concentrations were analyzed, and the results agreed well with those by the conventional liquid scintillation counting of electrolyzed combustion water of the samples. This showed that the method is practical and effective.We also developed an analytical method for non-exchangeable OBT as a combination of pre-treatment of dried samples with free water 3H and our newly developed analytical method for OBT. The repeated analysis of a grass sample with moderate 3H concentration had smaller variance of results for non-exchangeable OBT than for OBT. The sum of non-exchangeable and exchangeable OBT agreed well with OBT measured in the samples. The developed method was successfully applied to terrestrial and marine environmental samples with background 3H levels.