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The division's objectives are to promote the advancement of knowledge and understanding of the fundamental physical phenomena characterizing nuclear reactors and other nuclear systems. The division encourages research and disseminates information through meetings and publications. Areas of technical interest include nuclear data, particle interactions and transport, reactor and nuclear systems analysis, methods, design, validation and operating experience and standards. The Wigner Award heads the awards program.
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Become a knowledge manager at UWC 2024
The American Nuclear Society is now accepting applications for knowledge managers to work during the 2024 Utility Working Conference and Vendor Technology Expo. This year’s UWC, “Nuclear Momentum: Advancing Our Clean Energy Future,” will be held August 4–7, 2024, at the JW Marriott Marco Island Beach Resort on Marco Island, Fla.=
Zhongli Cai, Xifeng Li, Yosuke Katsumura, Osamu Urabe
Nuclear Technology | Volume 136 | Number 2 | November 2001 | Pages 231-240
Technical Paper | Radioactive Waste Management and Disposal | doi.org/10.13182/NT01-A3241
Articles are hosted by Taylor and Francis Online.
An understanding of the radiation-induced effects in groundwater is essential to evaluate the safe geological disposal of spent fuel. In groundwater, the bicarbonate ion is the predominant and common anion; this work investigated radiation-induced chemical reactions of (bi)carbonate aqueous solutions with steady-state irradiation and pulse radiolysis methods. Aqueous solutions of sodium (bi)carbonate as high as 50 mmoldm-3 were used. The formation of formate, oxalate, and H2O2 were measured under different conditions. A complete set of reaction steps and reliable kinetic data for the radiolysis of (bi)carbonate aqueous solutions at ionic strength close to the groundwater were proposed. Kinetic calculations were completed based on the proposed reaction steps and the kinetic data obtained in the present work. The results from the calculation are in good agreement with the experimental results. With these proposed reaction steps and kinetic data, computer simulation can be performed to predict the yield of radiolytic products of (bi)carbonate aqueous solutions as a function of irradiation time and used to evaluate the safety of geological disposal options of spent fuel.