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Glass strategy: Hanford’s enhanced waste glass program
The mission of the Department of Energy’s Office of River Protection (ORP) is to complete the safe cleanup of waste resulting from decades of nuclear weapons development. One of the most technologically challenging responsibilities is the safe disposition of approximately 56 million gallons of radioactive waste historically stored in 177 tanks at the Hanford Site in Washington state.
ORP has a clear incentive to reduce the overall mission duration and cost. One pathway is to develop and deploy innovative technical solutions that can advance baseline flow sheets toward higher efficiency operations while reducing identified risks without compromising safety. Vitrification is the baseline process that will convert both high-level and low-level radioactive waste at Hanford into a stable glass waste form for long-term storage and disposal.
Although vitrification is a mature technology, there are key areas where technology can further reduce operational risks, advance baseline processes to maximize waste throughput, and provide the underpinning to enhance operational flexibility; all steps in reducing mission duration and cost.
A. R. Massih
Nuclear Technology | Volume 205 | Number 7 | July 2019 | Pages 992-1001
Technical Note | doi.org/10.1080/00295450.2019.1568102
Articles are hosted by Taylor and Francis Online.
Oxidation of UO2 fuel under off-normal and normal reactor conditions occurs when fuel cladding fails, thereby allowing steam/water to enter the fuel rod. The steam/water will react with the fuel to produce UO2+x thus releasing hydrogen, with x standing for the amount of interstitial oxygen ions above the stoichiometric value.
In this technical note the impact of fuel oxidation on fission gas release (FGR) is modeled and discussed. The classical diffusion equation is used to describe migration and release of fission product gas (Xe) in UO2+x under time-varying postirradiation annealing conditions. We assume that the main quantity affected by fuel oxidation is the effective diffusivity of fission gas. Fuel oxidation enhances the diffusivity as a function of x in UO2+x in a parabolic fashion for 0.005 ≤ x ≤ 0.12 in the temperature range of 1000 ≤ T ≤ 1600 K. We first benchmark our model against an annealing test in which for x = 0.004 the Xe release fraction was measured as a function of time (temperature) during annealing. Furthermore, we apply the model to simulate a series of postirradiation annealing tests on UO2+x fuel, in which FGR fractions were measured for a given thermal ramp history in the range 0.00 ≤ x ≤ 0.66. The results of our computations in the range 0.004 ≤ x ≤ 0.20 show good agreement with measurements.