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Christmas Light
’Twas the night before Christmas when all through the house
No electrons were flowing through even my mouse.
All devices were plugged by the chimney with care
With the hope that St. Nikola Tesla would share.
Takeshi Tsukada, Keiju Takahashi
Nuclear Technology | Volume 162 | Number 2 | May 2008 | Pages 229-243
Technical Paper | First International Pyroprocessing Research Conference | doi.org/10.13182/NT08-A3951
Articles are hosted by Taylor and Francis Online.
In pyrometallugical reprocessing, the spent electrorefiner salt containing fission product (FP) elements may be purified by zeolite and reused. Batch-type absorption tests were conducted using one or two FP chlorides in a LiCl-KCl eutectic electrolyte in order to obtain absorption isotherms to fit to a Langmuir equation model. For the trivalent FP elements in the one-component or two-component systems, the FP-element uptake in the zeolite can be related to its concentration in the salt using a single Langmuir-type equation. In contrast, for monovalent and divalent FP elements, it was necessary to use three different Langmuir-type equations. Using these derived absorption equations and a stage concentration diagram, it was found that only a three-stage process is required to attain a decontamination factor of 50 for trivalent FP elements via a countercurrent multistage process.