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Glass strategy: Hanford’s enhanced waste glass program
The mission of the Department of Energy’s Office of River Protection (ORP) is to complete the safe cleanup of waste resulting from decades of nuclear weapons development. One of the most technologically challenging responsibilities is the safe disposition of approximately 56 million gallons of radioactive waste historically stored in 177 tanks at the Hanford Site in Washington state.
ORP has a clear incentive to reduce the overall mission duration and cost. One pathway is to develop and deploy innovative technical solutions that can advance baseline flow sheets toward higher efficiency operations while reducing identified risks without compromising safety. Vitrification is the baseline process that will convert both high-level and low-level radioactive waste at Hanford into a stable glass waste form for long-term storage and disposal.
Although vitrification is a mature technology, there are key areas where technology can further reduce operational risks, advance baseline processes to maximize waste throughput, and provide the underpinning to enhance operational flexibility; all steps in reducing mission duration and cost.
Ernst-Arndt Reinecke, Ahmed Bentaïb, Jürgen Dornseiffer, Daniel Heidelberg, Franck Morfin, Pascal Zavaleta, Hans-Josef Allelein
Nuclear Technology | Volume 196 | Number 2 | November 2016 | Pages 367-376
Technical Paper | doi.org/10.13182/NT16-4
Articles are hosted by Taylor and Francis Online.
Passive autocatalytic recombiners (PARs) have been installed inside light water reactor containments in many countries to remove hydrogen and, thus, to mitigate the combustion risk during a severe accident (SA). Due to the challenging SA boundary conditions, PARs are exposed to several deactivation risks during operation, which may cause a reduction of the hydrogen removal capacity. Such a deactivation may occur through different mechanisms and could in principle affect the start-up behavior up to the full loss of catalytic activity. To assess the interaction of PARs with the products of cable fires, a set of PAR catalyst samples has been introduced to the atmosphere of cable fire tests performed at Institut de Radioprotection et de Sûreté Nucléaire (IRSN), France. The subsequent surface analyses performed at Forschungszentrum Jülich (Germany) reveal a significant amount of carbon, chlorine (a constituent of polyvinyl chloride), zinc, and antimony (a flame retardant) on all catalyst samples compared to reference samples. The subsequent performance tests confirm that all catalyst sheets suffer a significant start-up delay of between 17 and 45 min compared to the reference samples. However, after burning off the soot deposition, the catalyst samples reach full conversion capacity and show immediate start-up behavior in a subsequent test. The present results clearly demonstrate the adverse effect of cable fire products on the efficiency of hydrogen conversion in a PAR. To further understand and quantify the impact of cable fire products and to assess their relevance for SA scenarios, further experimental as well as theoretical investigations are required. In particular, the combined influence of cable fire products and humidity, which has intentionally been omitted in the present study, should be investigated in the future due to the possible corrosive impact on the catalyst as well as the influence of humidity on the nature of the soot deposition.