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Argonne to investigate Pu chemistry to aid Hanford cleanup
Researchers at the Department of Energy’s Argonne National Laboratory are investigating the details of plutonium chemistry with the goal of aiding the cleanup of the Hanford Site in Washington state. For more than 40 years, reactors located at Hanford produced plutonium for America’s defense program, resulting in millions of gallons of liquid radioactive and chemical waste.
W. P. Poenitz
Nuclear Science and Engineering | Volume 57 | Number 4 | August 1975 | Pages 300-308
Technical Paper | doi.org/10.13182/NSE75-A15422
Articles are hosted by Taylor and Francis Online.
Absolute measurements of the capture cross section of197Au were carried out in the 400- to 3500-keV energy range. Ratios of the capture cross sections of 238U to 197Au were measured from 20 to 1200 keV. Values for σn,y(238U) were derived by utilizing evaluated and present data for σ n,γ(197Au). The time-of-flight technique and a large liquid scintillator were used for the detection of the prompt capture gamma rays, and the Grey Neutron Detector, the Black Neutron Detector, and a 6Li-glass detector were used for the measurement and monitoring of the neutron flux. The present results support previous measurements of the 238U capture cross section and resolve some existing discrepancies. The absolute values for the capture cross section of 197Au agree well with evaluated data and measurements reported relative to the 235U fission cross section.