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Latest News
Argonne to investigate Pu chemistry to aid Hanford cleanup
Researchers at the Department of Energy’s Argonne National Laboratory are investigating the details of plutonium chemistry with the goal of aiding the cleanup of the Hanford Site in Washington state. For more than 40 years, reactors located at Hanford produced plutonium for America’s defense program, resulting in millions of gallons of liquid radioactive and chemical waste.
J. E. Klein
Fusion Science and Technology | Volume 67 | Number 2 | March 2015 | Pages 416-419
Proceedings of TRITIUM 2013 | doi.org/10.13182/FST14-T42
Articles are hosted by Taylor and Francis Online.
The reduction in hydride absorption rate due to ”blanketing” can be explained in terms of a reduced hydrogen partial pressure in the bed due to the accumulation of inerts (i.e. non-hydrogen isotopes) in the bed void volume. Literature results show reduced absorption rates when protium for bed absorption contains helium with low-end inert compositions in the 0.6 to 1% range. A hydride bed containing 9.66 kg of LaNi4.25Al0.75 (LANA0.75) metal hydride - a nominal capacity of 1400 STP-L, was cycled repeatedly to decrepitate the hydride material into smaller particles for bed strain measurement. The hydride cycles added and removed nominally 1000 to 1100 STP-L of protium per hydride cycle. Consistent and repeatable absorptions results were observed for different absorption cycles. During one of the absorption tests, slower absorption results were obtained due to the use of typical grade (500 ppm inerts), instead of research grade, protium which blanketed the bed. The impact of 0.05% inerts in protium on bed absorption rate is shown and explained in terms of an increase in inert partial pressure as the bed was loaded.