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2025 ANS Winter Conference & Expo
November 9–12, 2025
Washington, DC|Washington Hilton
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OECD NEA meeting focuses on irradiation experiments
Members of the OECD Nuclear Energy Agency’s Second Framework for Irradiation Experiments (FIDES-II) joint undertaking gathered from September 29 to October 3 in Ketchum, Idaho, for the technical advisory group and governing board meetings hosted by Idaho National Laboratory. The FIDES-II Framework aims to ensure and foster competences in experimental nuclear fuel and structural materials in-reactor experiments through a diverse set of Joint Experimental Programs (JEEPs).
Naoki Yoshida, Takuya Ohno, Yuki Amano, Ryoichiro Yoshida, Hitoshi Abe, Yuichi Yamane
Nuclear Technology | Volume 210 | Number 10 | October 2024 | Pages 1999-2007
Note | doi.org/10.1080/00295450.2024.2306688
Articles are hosted by Taylor and Francis Online.
A malfunction of the cooling system of high-level liquid waste (HLLW) and the failure of countermeasures may lead to the evaporation to dryness due to the loss of cooling functions (EDLCF) of the HLLW. In the EDLCF, ruthenium (Ru) can be released at a greater fraction to the initial amount than the other elements in HLLW by forming gaseous Ru. It is important to identify the chemical form of the released gaseous Ru to achieve a comprehensive understanding of the events impacting the source term assessment of Ru in this accident, such as particle formation, gas absorption, and deposition on migration pathways.
In this study, we observed the ultraviolet/visible spectroscopy of the off-gas generated during the heating of a HLLW simulant. Employing a program that allows for the separation and quantification of known components within the spectrum [ruthenium tetroxide (RuO4), nitrogen dioxide, and nitric acid], we attempted to analyze the composition of gaseous Ru within the generated off-gas. Our findings revealed RuO4 as the main component of the gaseous Ru in the off-gas after comparing the total amount of released Ru and the RuO4 released amount obtained via spectroscopic analysis.
