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General Kenneth Nichols and the Manhattan Project
Nichols
The Oak Ridger has published the latest in a series of articles about General Kenneth D. Nichols, the Manhattan Project, and the 1954 Atomic Energy Act. The series has been produced by Nichols’ grandniece Barbara Rogers Scollin and Oak Ridge (Tenn.) city historian David Ray Smith. Gen. Nichols (1907–2000) was the district engineer for the Manhattan Engineer District during the Manhattan Project.
As Smith and Scollin explain, Nichols “had supervision of the research and development connected with, and the design, construction, and operation of, all plants required to produce plutonium-239 and uranium-235, including the construction of the towns of Oak Ridge, Tennessee, and Richland, Washington. The responsibility of his position was massive as he oversaw a workforce of both military and civilian personnel of approximately 125,000; his Oak Ridge office became the center of the wartime atomic energy’s activities.”
Javiera Cervini-Silva
Nuclear Technology | Volume 210 | Number 8 | August 2024 | Pages 1487-1495
Note | doi.org/10.1080/00295450.2023.2295152
Articles are hosted by Taylor and Francis Online.
Bentonites are natural reservoirs of various elements and are of interest because they are sources of thorium and uranium, which are transition elements that provide nuclear energy. The objective of this work was to study the plausible association(s) of these elements with other transition elements of interest. The contents of 18 transition elements (cerium, cobalt, chromium, copper, iron, hafnium, lanthanum, manganese, molybdenum, neodymium niobium, nickel, tantalum, thorium, uranium, vanadium, yttrium, zinc, and zirconium) in 38 bentonites determined experimentally by X-ray fluorescence spectroscopy (XRF) were analyzed.
The contents of the elements were plotted in (x,y) graphs and then fitted to polynomial functions (orders 1 through 6). According to the coefficient of determination (r2: 0.5 ≤ r2 strong, 0.3 ≤ r2 ≤ 0.5 medium, and r2 ≤ 0.3 weak), the contents of thorium, uranium, niobium, and nickel related strongly, thus the presence of niobium and nickel served to predict the presence of detectable concentrations of thorium and uranium. The equations showing higher r2 values were
1. {Th} = 1e-6{Nb}5 − 3e-4{Nb}4 + 1.9e-2{Nb}3 − 5.4e-1{Nb}2 + 7.3{Nb} − 6.3, r2 = 0.53.
2. {Th} = −3e-8{Nb}6 + 9e-6{Nb}5 − 1e-3{Nb}4 + 4.7e-2{Nb}3 − 1.1{Nb}2 + 11.5{Nb} − 16, r2 = 0.54.
3. {Th} = 5e-6{Ni}4 − 1.5e-3{Ni}3 − 1.5e-1{Ni}2 − 5.8{Ni} + 9e+1, r2 = 0.49.
4. {Th} = −7e-8{Ni}5 + 3e-5{Ni}4 − 5.1e-3{Ni}3 + 3.4e-1{Ni}2 − 9.5{Nb} + 1e+2, r2 = 0.56.
5. {Th} = 2e-9{Ni}6 − 8e-7{Ni}5 + 2e-4{Ni}4 − 1.5e-2{Ni}3 − 7e-1{Ni}2 − 1e+1{Ni} + 1e+1, r2 = 0.60.
6. {Th} = −1e-4{U}5 + 1.3e-2{U}4 − 4.3e-1{U}3 + 5.7e-1{U}2 − 2e+1{U} + 5e+1, r2 = 0.54.
7. {Th} = 6e-6{U}6 − 9e-4{U}5 + 4.5e-2{U}4 − 1.1{U}3 + 1e+1{U}2 − 5e+1{U} + 1e+2, r2 = 0.64.
8. {U} = 8e-6{Nb}4 − 1.2e-3{Nb}3 + 4.8e-2{Nb}2 − 4.3e-1{Nb} + 6.8, r2 = 0.48.
9. {U} = 2e-7{Nb}5 − 4e-5{Nb}4 + 2.8e-3{Nb}3 − 7.6e-2{Nb}2 + 1.1{Nb} + 1.9, r2 = 0.5.
10. {U} = 1e-8{Nb}6 − 3e-6{Nb}5 + 2e-4{Nb}4 − 8e-3{Nb}3 + 1.3e-1{Nb}2 − 5.4e-1{Nb} + 5.4, r2 = 0.51.
11. {U} = 1.8e-1{Th} + 2.6, r2 = 0.49; {U} = 1.7e-3{Th}2 − 2.9e-2{Th} + 6.3, r2 = 0.60.
12. {U} = 2e-5{Th}3 − 1.7e-3{Th}2 + 1.4e-1{Th} + 4.5, r2 = 0.58; {U} = −5e-7{Th}4 + 2e-4{Th}3 − 1.5e-2{Th}2 + 5.5e-1{Th} + 1.5, r2 = 0.6.
13. {U} = −7e-9{Th}5 + 2e-6{Th}4 − 1e-4{Th}3 − 3e-4{Th}2 + 2.7e-1{Th} + 2.9, r2 = 0.6.
14. {U} = 2e-9{Th}6 − 8e-7{Th}5 + 1e-4{Th}4 − 8.1e-3{Th}3 − 2.4e-1{Th}2 + 15, r2 = 0.65.
This study provided a joint experimental and theoretical approach to optimize the recovery of thorium and uranium and to save invaluable onsite and off-site natural resources and work time. The findings might expand on other studies reporting the quantification of transition metals on bentonite matrices. For instance, the concentrations of nickel reported in studies using bench techniques could serve as the basis to calculate the contents of thorium.
