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Glass strategy: Hanford’s enhanced waste glass program
The mission of the Department of Energy’s Office of River Protection (ORP) is to complete the safe cleanup of waste resulting from decades of nuclear weapons development. One of the most technologically challenging responsibilities is the safe disposition of approximately 56 million gallons of radioactive waste historically stored in 177 tanks at the Hanford Site in Washington state.
ORP has a clear incentive to reduce the overall mission duration and cost. One pathway is to develop and deploy innovative technical solutions that can advance baseline flow sheets toward higher efficiency operations while reducing identified risks without compromising safety. Vitrification is the baseline process that will convert both high-level and low-level radioactive waste at Hanford into a stable glass waste form for long-term storage and disposal.
Although vitrification is a mature technology, there are key areas where technology can further reduce operational risks, advance baseline processes to maximize waste throughput, and provide the underpinning to enhance operational flexibility; all steps in reducing mission duration and cost.
Tae-Hoon Lee, Spencer Menlove, Howard O. Menlove, Hee-Sung Shin, Ho-Dong Kim
Nuclear Technology | Volume 206 | Number 7 | July 2020 | Pages 984-992
Regular Technical Paper | doi.org/10.1080/00295450.2020.1743598
Articles are hosted by Taylor and Francis Online.
The transuranic (TRU) ingot is considered to be the most prominent target material of pyroprocessing in terms of safeguards since it contains almost all of the Pu of the feed spent fuel. Due to the high density, excessively high neutron emission rates, and high neutron multiplication of the U/TRU ingot, it is impractical to apply gamma-ray spectroscopy or neutron coincidence counting techniques to the quantification of the Pu content of the U/TRU ingot. Since the passive neutron albedo reactivity (PNAR) technique is known to be sensitive to the total fissile mass of target material and the uncertainty of its singles Cd ratio is independent of the accidental coincidence coming from the high neutron emission rate, the capability of the PNAR technique for the quantification of the Pu content of the U/TRU ingot has been investigated using the MCNPX code with a spent fuel library with 81 different cases of various kinds of initial enrichment, burnup, and cooling time. The MCNPX simulation results for the Cd ratio versus Pu content of the U/TRU ingot show the maximum error in the Pu mass between the linear fit and the real Pu content in the U/TRU ingot is 2.14% for 4.5 wt% initial enrichment cases. The results of this study show that the PNAR technique can be one possible method for the direct nondestructive assay for the Pu of the U/TRU ingot.