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High-temperature plumbing and advanced reactors
The use of nuclear fission power and its role in impacting climate change is hotly debated. Fission advocates argue that short-term solutions would involve the rapid deployment of Gen III+ nuclear reactors, like Vogtle-3 and -4, while long-term climate change impact would rely on the creation and implementation of Gen IV reactors, “inherently safe” reactors that use passive laws of physics and chemistry rather than active controls such as valves and pumps to operate safely. While Gen IV reactors vary in many ways, one thing unites nearly all of them: the use of exotic, high-temperature coolants. These fluids, like molten salts and liquid metals, can enable reactor engineers to design much safer nuclear reactors—ultimately because the boiling point of each fluid is extremely high. Fluids that remain liquid over large temperature ranges can provide good heat transfer through many demanding conditions, all with minimal pressurization. Although the most apparent use for these fluids is advanced fission power, they have the potential to be applied to other power generation sources such as fusion, thermal storage, solar, or high-temperature process heat.1–3
Berkan Çetinkaya, Hüseyin Tel, Ahmet Yaylı
Nuclear Technology | Volume 206 | Number 5 | May 2020 | Pages 717-727
Technical Paper | doi.org/10.1080/00295450.2019.1686939
Articles are hosted by Taylor and Francis Online.
(ThxCe1-x)O2 microspheres (x = 0.50, 0.75, and 0.95) prepared by sol-gel microsphere technique were compacted to pellets. The sintering kinetics, diffusion mechanism, and activation energy of the (ThxCe1-x)O2 pellets were investigated by dilatometry for 1100°C, 1200°C, and 1300°C. The rate controlling sintering method, one of the most sensitive methods, was chosen to investigate the sintering kinetics. The pellets were heated with a rate of 10°C/min and were held for 10 h at the above mentioned temperatures under isothermal conditions.
The activation energies for the (Th0.50Ce0.50)O2, (Th0.75Ce0.25)O2, and (Th0.95Ce0.05)O2 pellets were calculated as 305, 315, and 419 kJ·mol−1, respectively. In the experiments, green densities of the mixed-oxide pellets were determined as 45% to 47% of the theoretical density for all of the studied ratios. Sintering densities reached up to 94% of theoretical density after sintering at 1300°C. Scanning electron microscopy images of the pellets were taken.
