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Undeclared uranium hitches a ride on cobalt exports from Congo, study says
Philippe (left) and Manzuk quantified the amount of uranium that has been exported from the DRC in cobalt shipments or left behind in the environment. (Photo: Joel Hallberg/UW–Madison)
Researchers at the University of Wisconsin–Madison and Princeton University have published a study in Nature Communications that calls attention to a blind spot in nuclear nonproliferation: The Democratic Republic of the Congo (DRC) has exported thousands of metric tons of uranium, and there is no accounting for where it has gone.
In partnership with Lighthouse Reports and the Financial Times, UW–Madison nuclear engineering professor and nuclear security expert Sébastien Philippe and Ryan Manzuk, a geologist and research fellow in Philippe’s group and at Princeton, conducted the study using countrywide mineralization and geochemical data.
Staffan Qvist
Nuclear Technology | Volume 190 | Number 1 | April 2015 | Pages 11-27
Technical Paper | Fission Reactors | doi.org/10.13182/NT14-30
Articles are hosted by Taylor and Francis Online.
In this study, the characteristics of changes in reactivity due to increasing burnup of uranium-fueled fast reactors are analyzed. A new classification system for nuclear reactor cores based on their uncontrolled tendency for reactivity changes during burnup was introduced and the design-optimization strategy for any fast reactor core aimed at a minimized reactivity swing is outlined. The 235U feed-fuel enrichment level that minimizes the burnup reactivity swing of a sodium-cooled metallic-fueled core is 10% to 12.5% for an average target fuel burnup of 1% to 20% FIMA (fission of initial metal atom). The higher the target burnup of the system, the lower the feed-fuel enrichment level that minimizes swing. The minimum attainable swing for a 125-MW(thermal) metallic-fueled sodium-cooled core is found to be ∼200 pcm for 5% FIMA burnup and increases to ∼800 pcm for a system aiming at 10% FIMA. In general, if the target discharge burnup is doubled, the minimum attainable burnup reactivity swing quadruples. Any optimized minimum reactivity swing core will form a positive parabolic uncontrolled reactivity trajectory with burnup, where the beginning of cycle and end of cycle reactivities are equal. Uranium-fueled fast cores with minimized burnup reactivity swing are net consumers of fissile material, with a fissile conversion ratio in the range of 0.7 to 0.9.