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Smarter waste strategies: Helping deliver on the promise of advanced nuclear
At COP28, held in Dubai in 2023, a clear consensus emerged: Nuclear energy must be a cornerstone of the global clean energy transition. With electricity demand projected to soar as we decarbonize not just power but also industry, transport, and heat, the case for new nuclear is compelling. More than 20 countries committed to tripling global nuclear capacity by 2050. In the United States alone, the Department of Energy forecasts that the country’s current nuclear capacity could more than triple, adding 200 GW of new nuclear to the existing 95 GW by mid-century.
B.-G. Brodda, D. Heinen
Nuclear Technology | Volume 34 | Number 3 | August 1977 | Pages 420-427
Technical Paper | Chemical Processing | doi.org/10.13182/NT77-A31807
Articles are hosted by Taylor and Francis Online.
The radiolytic load of the 30 vol% tributylphosphate-n-paraffin extractant to be used in the Jülich Pilot Plant for Thorium Element Reprocessing facility for reprocessing thorium high-temperature reactor (THTR) fuel elements with high burn-up values (85 000 MWd/MT of heavy-metal atoms) was calculated. At a radioactivity level of ∼2000 Ci/ℓ, the effective beta-particle power density of the feed solution ranges up to 15 W · ℓ−1. Most of the energy absorbed by the extractant is due to beta radiation (99%). About 1% originates from gamma radiation; contributions from alpha-particle emitters are negligible. The calculations consider the geometric parameters of the applied mixer-settler and the operational parameters of the flowsheet. The highest exposure expected will be ∼0.2 Wh · ℓ−1 · pass−1 when reprocessing fuel with 85 000 MWd/MT burnup after a cooling time of 100 days. For an easier comparison of the calculated value with other reported values, a coefficient is introduced describing the specific exposure of the extractant in terms of energy absorption per hour of passing through the contactor at a power density of 1 W· ℓ−1 in the feed solution. This coefficient is independent of such individual flowsheet conditions as heavy-metal concentration or power density in the feed solution. Comparison of calculated data with other reported data for THOREX and PUREX reprocessing runs exhibits only about a four-fold specific load of the extractant in case of reprocessing high-burned-up THTR fuel with respect to low-enriched low-burned-up light water reactor fuel. This underproportional increase is due to the specific fission-product spectrum of the investigated THTR fuel arising in the course of its reactor residence time.