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Glass strategy: Hanford’s enhanced waste glass program
The mission of the Department of Energy’s Office of River Protection (ORP) is to complete the safe cleanup of waste resulting from decades of nuclear weapons development. One of the most technologically challenging responsibilities is the safe disposition of approximately 56 million gallons of radioactive waste historically stored in 177 tanks at the Hanford Site in Washington state.
ORP has a clear incentive to reduce the overall mission duration and cost. One pathway is to develop and deploy innovative technical solutions that can advance baseline flow sheets toward higher efficiency operations while reducing identified risks without compromising safety. Vitrification is the baseline process that will convert both high-level and low-level radioactive waste at Hanford into a stable glass waste form for long-term storage and disposal.
Although vitrification is a mature technology, there are key areas where technology can further reduce operational risks, advance baseline processes to maximize waste throughput, and provide the underpinning to enhance operational flexibility; all steps in reducing mission duration and cost.
Shunsuke Uchida, Masanori Naitoh, Hidetoshi Okada, Hiroaki Suzuki, Soji Koikari, Seiichi Koshizuka, Derek H. Lister
Nuclear Technology | Volume 180 | Number 1 | October 2012 | Pages 65-77
Technical Paper | Thermal Hydraulics | doi.org/10.13182/NT12-A14519
Articles are hosted by Taylor and Francis Online.
A modified six-step evaluation procedure has been proposed to evaluate local wall thinning due to flow-accelerated corrosion (FAC). In step 1, the one-dimensional (1-D) distribution of flow turbulence and the temperature along pipes in cooling systems were analyzed with a 1-D system simulation code to obtain approximate mass transfer coefficients at structure surfaces, prior to using a three-dimensional (3-D) computational fluid dynamics (CFD) code for precise flow turbulence analysis of the major parts. In step 2, corrosive conditions were calculated with a N2H4-O2 reaction analysis code. In step 3, high FAC risk zones were determined for further evaluation for wall thinning rates, based on five parameters: temperature, pH, oxygen concentration, mass transfer coefficient, and chromium content. Then, in step 4, the 3-D CFD code was used to calculate precise mass transfer coefficients at the high FAC risk zones. In step 5, the wall thinning rates were calculated using a coupled model of electrochemical analysis and oxide layer growth analysis by applying the corrosive conditions and the mass transfer coefficients. Finally, in step 6, the residual lifetime of the pipes and the applicability of countermeasures against FAC were evaluated.This paper introduces procedures for determining major FAC parameters and evaluation procedures for high FAC risk zones by synthesizing the parameters in step 3. The procedures for determination of high FAC risk zones in a pressurized water reactor secondary cooling system are also demonstrated.