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Why should safeguards by design be a global effort?
Jeremy Whitlock
I can’t think of a more exciting time to be working in nuclear, with the diversity of advanced reactor development and increasing global support for nuclear in sustainable energy planning. But we can’t lose sight of the need to plan for efficient international safeguards at the same time.
Global nuclear deployment has been underpinned since 1970 by the Treaty on the Non-Proliferation of Nuclear Weapons (NPT), making it a key customer requirement for governments to demonstrate unequivocally that the technology is not being misused for weapons development.
The International Atomic Energy Agency (IAEA) has helped verify this commitment for more than 50 years, but it has never safeguarded many of the advanced reactors (and related fuel cycle processes) being developed today.
Masaumi Nakahara, Tsutomu Koizumi, Kazunori Nomura
Nuclear Technology | Volume 174 | Number 1 | April 2011 | Pages 77-84
Technical Paper | Chemical Reprocessing | doi.org/10.13182/NT11-A11681
Articles are hosted by Taylor and Francis Online.
A crystal purification process consisting of sweating and melt filtration was developed to improve decontamination factors (DFs) of fission product impurities from uranyl nitrate hexahydrate (UNH) crystal recovered from a dissolver solution of irradiated fast reactor core fuel. Batch experiments on the sweating and melt filtration processes were carried out at 56 to 80°C. Although the DFs of solid impurities such as Cs and Ba remain the same in the sweating process, those of liquid impurities such as Zr, Nb, Ru, Ce, and Eu were 2.32, 2.40, 2.50, 2.45, and 2.60 at 60°C. On the other hand, the DF of Pu for the UNH crystal slightly increased to 1.25 at 60°C. Because Pu incorporated the UNH crystal in both the solid impurities such as Cs2Pu(NO3)6 and in the liquid impurities, Pu in the liquid fraction was removed by the sweating operation. Decontamination of liquid impurities was effective with sweating time and with a rise in sweating temperature. In the melt filtration process, 0.45- to 5.0-m-diam filters were used for the separation of the molten UNH crystal. The DF of Ba was approximately ten times as high as the crude crystal with 0.45- to 5.0-m-diam filters. The particle size of Pu and Cs formed as Cs2Pu(NO3)6 was quite small. As a proof of this, although the decontamination of Pu and Cs was not effective with a 5.0-m-diam filter, their DFs rose 2.7 times using a 0.45-m-diam filter.