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Glass strategy: Hanford’s enhanced waste glass program
The mission of the Department of Energy’s Office of River Protection (ORP) is to complete the safe cleanup of waste resulting from decades of nuclear weapons development. One of the most technologically challenging responsibilities is the safe disposition of approximately 56 million gallons of radioactive waste historically stored in 177 tanks at the Hanford Site in Washington state.
ORP has a clear incentive to reduce the overall mission duration and cost. One pathway is to develop and deploy innovative technical solutions that can advance baseline flow sheets toward higher efficiency operations while reducing identified risks without compromising safety. Vitrification is the baseline process that will convert both high-level and low-level radioactive waste at Hanford into a stable glass waste form for long-term storage and disposal.
Although vitrification is a mature technology, there are key areas where technology can further reduce operational risks, advance baseline processes to maximize waste throughput, and provide the underpinning to enhance operational flexibility; all steps in reducing mission duration and cost.
S. R. Boddu, V. R. Gutti, R. M. Meyer, T. K. Ghosh, R. V. Tompson, S. K. Loyalka
Nuclear Technology | Volume 173 | Number 3 | March 2011 | Pages 318-326
Technical Paper | Miscellaneous | doi.org/10.13182/NT11-A11665
Articles are hosted by Taylor and Francis Online.
Nanoparticles can form during nuclear accidents as well as during normal nuclear reactor operations and can be both radioactive and nonradioactive. It is important to understand particle size characteristics, transport properties, and deposition in order to better predict the behaviors of, and effects due to, these particles in a reactor. Fission products can deposit (adsorb/absorb) on the graphite dust in the core [an amount of carbon dust is present in the Pebble Bed Modular Reactor (PBMR) because of graphite sphere abrasion] and can also be carried by the helium flow (together with some dust). Generating nanoparticles of desired shape, size, and purity for experimental purposes is difficult, and hence, there is a need for new and refined synthesis techniques. Nanoparticle generation using high-voltage electric sparks has become a technique of interest for a wide range of conducting materials, and particles with sizes ranging from a few nanometers up to microns have been generated in this manner in an aerosol state. Our purpose in this paper is to report on the generation, collection, and characterization of carbon nanoparticles. We have used a spark generator and a thermophoretic deposition cell, as well as environmental scanning electron microscopy, transmission electron microscopy, and scanning mobility particle spectrometry. We have explored a number of experimental conditions, and we find that one can generate and effectively collect test particles with a variety of different useful characteristics. We also discuss some computational fluid dynamics simulations of particle deposition in the thermophoretic deposition cell.