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Remembering Charles E. Till
Charles E. Till
Charles E. Till, an ANS member since 1963 and Fellow since 1987, passed away on March 22 at the age of 89. He earned bachelor’s and master’s degrees from the University of Saskatchewan and a Ph.D. in nuclear engineering from Imperial College, University of London. Till initially worked for the Civilian Atomic Power Department of the Canadian General Electric Company, where he was the physicist in charge of the startup of the first prototype CANDU reactor in Canada.
Till joined Argonne National Laboratory in 1963 in the Applied Physics Division, where he worked as an experimentalist in the Fast Critical Experiments program. He then moved to additional positions of increasing responsibility, becoming division director in 1973. Under his leadership, the Applied Physics Division established itself as one of the elite reactor physics organizations in the world. Both the experimental (critical experiments and nuclear data measurements) and nuclear analysis methods work were internationally recognized. Till led Argonne’s participation in the International Nuclear Fuel Cycle Evaluation (INFCE), and he was the lead U.S. delegate to INFCE Working Group 5, Fast Breeders.
Yung-Zun Cho, Gil-Ho Park, Han-Su Lee, In-Tae Kim, Dae-Seok Han
Nuclear Technology | Volume 171 | Number 3 | September 2010 | Pages 325-334
Technical Paper | Pyro 08 Special / Reprocessing | doi.org/10.13182/NT09-7
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As an alternative to conventional Group I and II separation methods (such as adding a chemical agent and ion exchange), melt crystallization processes, zone freezing, and layer melt crystallization were tested for the separation (or concentration) of cesium and strontium fission products in a LiCl waste salt generated from an electrolytic reduction process of a spent oxide fuel. In these melt crystallization processes, impurities (CsCl and SrCl2) are concentrated in a small fraction of the LiCl salt by the solubility difference between the melt phase and the crystal phase. As experimental variables, initial molten salt temperature, crucible rising velocity in the zone freezing case, and cooling air flow rate in the layer crystallization case were used. In the zone freezing process, although the operating time is long (1.7 mm/h of crucible rising velocity) when assuming a LiCl salt reuse rate of 90 wt%, >90% separation efficiency for both CsCl and SrCl2 was shown. In the layer crystallization process, the crystal growth rate strongly affects the crystal structure and therefore the separation efficiency. At a 25 to 30 [script l]/min cooling air flow rate, 700 to 710°C initial molten salt temperature, and <5 g/min crystal growth rate, the separation efficiency of both CsCl and SrCl2 exceeded 90% by the layer crystallization process, assuming a LiCl salt reuse rate of 90 wt%.