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Conference Spotlight
2025 ANS Winter Conference & Expo
November 9–12, 2025
Washington, DC|Washington Hilton
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A wave of new U.S.-U.K. deals ahead of Trump’s state visit
President Trump will arrive in the United Kingdom this week for a state visit that promises to include the usual pomp and ceremony alongside the signing of a landmark new agreement on U.S.-U.K. nuclear collaboration.
Thi Thanh Thuy Nguyen, Kwang Soon Ha, Jin Ho Song, Sung Il Kim
Nuclear Science and Engineering | Volume 193 | Number 8 | August 2019 | Pages 916-925
Technical Paper | doi.org/10.1080/00295639.2019.1574118
Articles are hosted by Taylor and Francis Online.
A new empirical model is proposed for estimating the amount of volatile iodine in an aqueous phase. The volatile iodine concentration is estimated for highly irradiated CsI solutions in which the pH of the solution changes. The reaction of CsI solution with water radiolysis products is not balanced because radiolysis products are continuously produced under irradiation. Thus the kinetic of the chemical equation is important to determine iodine behavior in a CsI solution. An empirical model for the kinetic equation including the oxidation and reduction reaction is proposed. The proposed model was validated with a wide range of experimental data. A comparison of the experiments and predictions by the model indicated that the predicted volatile iodine from CsI solution with a concentration of 10−3 to 10−4 M was in good agreement. For 10−5 M CsI solution, the predicted iodine concentration was much smaller than experimental data due to the fact that I− was rapidly converted to IO3−.