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Spent fuel recycling and conditioning topic of U.S.-Japan meeting
Officials with the Department of Energy’s Office of Environmental Management discussed spent nuclear fuel recycling and conditioning with counterparts from Japan during the 13th U.S.-Japan Technical Meeting of the Civil Nuclear Energy Research and Development Working Group, held recently in Santa Fe, N.M.
C. D. Bowman, E. G. Bilpuch, D. C. Bowman, A. S. Crowell, C. R. Howell, K. McCabe, G. A. Smith, A. P. Tonchev, W. Tornow, V. Violet, R. B. Vogelaar, R. L. Walter, J. Yingling
Nuclear Science and Engineering | Volume 161 | Number 1 | January 2009 | Pages 68-77
Technical Paper | doi.org/10.13182/NSE161-68
Articles are hosted by Taylor and Francis Online.
The results of two experiments combined show that the diffusion length D for thermal neutrons in the graphite studied is 24% larger than expected from classical experiments and that the boron equivalent absorption is smaller than expected and consistent with zero. Taken together, the results indicate a reduction in parasitic thermal neutron absorption in heterogeneous graphite reactors by about 30%. The first experiment measured the z-dependence of thermal neutron flux in a column of 12 t of granular graphite with a neutron source at the bottom. A second measurement was made by pulsing the column with a neutron source at its center and measuring the neutron decay rate as a function of time after a pure exponential decay had been established. The diffusion coefficient D adjusted to a density of 1.60 g/cm3 is 1.05 ± 0.03 cm compared with the commonly accepted value of 0.85 ± 0.013 cm. The absorption in our graphite owing to impurities was found to be <10% of that from carbon alone. The parameter a/D that measures neutron loss was determined to be 0.000235 ± 0.000026 cm-2 for a density of 1.60 g/cm3 and may be compared with the commonly accepted value of 0.000340. The performance of graphite thermal spectrum reactors constructed using our graphite would be significantly enhanced over present expectations because neutron loss to graphite is a major factor in the neutron economy of graphite-moderated thermal reactors.