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J. J. KEPES, L. A. MIKOLEIT, R. G. SERENKA
Nuclear Science and Engineering | Volume 14 | Number 1 | September 1962 | Pages 11-16
Technical Paper | doi.org/10.13182/NSE62-A26194
Articles are hosted by Taylor and Francis Online.
Differential measurements of the epicadmium and total U238 radiative capture have been obtained in thin natural uranium-niobium plates and compared to several theoretical models. These fuel elements were located in Zircaloy-2 boxes, which in turn were placed in a light water moderated critical assembly at ambient temperatures. A Monte Carlo calculation with the assumption of a smooth 3.3 b contribution predicted the spatial epicadmium activation through a natural uranium fuel plate positioned in the center of the Zircaloy-2 box. It was observed that the integrated epicadmium U238 radiative capture in the end fuel plate of the Zircaloy-2 box was 1.27 times the capture in the center fuel plate. This sharp end-to-center dipping was due to a water channel located next to the fuel box. An analytic calculation based on the thin resonance theory of Stein gave a value of 1.16 for this end-to-center ratio. The experimental integrated values for ρ28, the ratio of epicadmium to thermal captures, were 0.893 ± 0.009 in the center fuel plate, 0.765 ± 0.014 in the second from the end plate, and 0.851 ± 0.011 in the end plate. The value of ρ28 obtained using a diffusion theory approximation for these plates was 4.7%, 7.5%, and 21.7% below experiment. The prediction in the end plate was improved when the Stein theory was utilized to calculate the resonance capture.