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Washington, DC|Washington Hilton
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Leading the charge: INL’s role in advancing HALEU production
Idaho National Laboratory is playing a key role in helping the U.S. Department of Energy meet near-term needs by recovering HALEU from federal inventories, providing critical support to help lay the foundation for a future commercial HALEU supply chain. INL also supports coordination of broader DOE efforts, from material recovery at the Savannah River Site in South Carolina to commercial enrichment initiatives.
W. Breitung, K. O. Reil
Nuclear Science and Engineering | Volume 101 | Number 1 | January 1989 | Pages 26-40
Technical Paper | doi.org/10.13182/NSE89-A23592
Articles are hosted by Taylor and Francis Online.
Newly developed in-pile techniques were used to measure the saturation vapor pressure of pure UO2.01, reactor grade UO2.08, and reactor grade (U0.77Pu0.23)O2.09 between 2000 and 3700 kJ/kg. The results for all three fuel types can be described by log Psat (z) = -9.7652 + 8.0934 × 10-3z - 2.0515 × 10-6z2 + 1.9013 × 10-10z3 with z = h-h298 in kilojoules per kilogram and psat in megapascals. The data were converted to the pressure-temperature format and compared to earlier out-of-pile vapor pressure measurements. All out-of-pile measurements that were performed close to a vapor-liquid equilibrium state agree very well with the in-pile results. The following relation is proposed for the p-T saturation line of liquid UO2: log psat (T) = 15.961 - 26974/T - 2.7600 log T, with psat in megapascals and T in degrees kelvin. Because no significant differences were found for all three fuel types investigated, the same saturation vapor pressure is recommended for liquid-metal fast breeder reactor (LMFBR) typical (U,Pu) mixed oxides under LMFBR core disassembly conditions.
