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Perpetual Atomics, QSA Global produce Am fuel for nuclear space power
U.K.-based Perpetual Atomics and U.S.-based QSA Global claim to have achieved a major step forward in processing americium dioxide to fuel radioisotope power systems used in space missions. Using an industrially scalable process, the companies said they have turned americium into stable, large-scale ceramic pellets that can be directly integrated into sealed sources for radioisotope power systems, including radioisotope heater units (RHUs) and radioisotope thermoelectric generators (RTGs).
Y. L. Sandler, R. H. Kunig
Nuclear Science and Engineering | Volume 64 | Number 4 | December 1977 | Pages 866-874
Technical Paper | doi.org/10.13182/NSE77-A14502
Articles are hosted by Taylor and Francis Online.
The solubility of a nickel ferrite, NixFe3-xO4, as a model substance for deposits forming on the cladding of nuclear fuel elements of pressurized water reactors is determined in aqueous solutions of primary coolant composition at different pH and hydrogen concentrations, in the temperature region from 230 to 330°C. The temperature coefficient of solubility changes from negative to positive at about pH 7 with increasing pH. The data agree reasonably well with those of Sweeton and Baes for magnetite, considering the lower iron activity in the nickel ferrite. The solubility of nickel is generally lower than that which corresponds to a congruent solution and goes through a minimum near pH 7.4. The iron solubility appears to depend on the one-third power of the hydrogen concentration in solution in the region from 20 to 100 cm3 H2/kg H2O, as expected. Preliminary results, however, indicate that at lower hydrogen concentrations, the dependence on the hydrogen concentration can decrease, possibly due to the formation of cation vacancies.