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DOE, PNNL, and Commerce Dept. collaborate on Ra-226 recovery
PNNL’s Jamin Trevino works with a capsule containing Ra-226. (Photo: Jamin Trevino/PNNL)
A collaboration between the Department of Energy’s Office of Isotope R&D and Production and the Department of Commerce’s National Institute of Standards and Technology has recovered large quantities of radium-226—valued for its use in medical radioisotope production—from radiological waste stored at NIST facilities. Ra-226 is an important element in developing therapies for patients fighting cancer.
R. H. Chen, M. L. Corradini, G. H. Su, S. Z. Qiu
Nuclear Science and Engineering | Volume 174 | Number 1 | May 2013 | Pages 46-59
Technical Paper | doi.org/10.13182/NSE12-22
Articles are hosted by Taylor and Francis Online.
In the present study, we propose a new fragmentation criterion for the explosion phase to take account of the effect of partial fuel melt solidification on the rapid fragmentation process. This new criterion judges whether or not the explosive fragmentation can occur by comparing the impact stress induced by vapor film collapse and water jet impingement with the fracture toughness of the corium crust layer. The fragmentation criterion was incorporated into the revised Thermal EXplosion Analysis Simulation (TEXAS) fuel-coolant-interaction (FCI) model TEXAS-VI and combined with the previously proposed fuel particle solidification model and the fragmentation criterion for the mixing phase. TEXAS-VI was compared to KROTOS alumina test K-44 and corium tests K-52 and K-53, and good agreement was obtained. The simulation results indicate that TEXAS-VI has the capability to consider the effect of partial solidification for both the mixing and the explosion phases of the FCI process and can capture the effect of fuel solidification, which reduces corium-water explosion energetics. Experiments K-52 and K-53 also demonstrate the ability of TEXAS-VI to model the effects of ambient pressure on energetics.