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Fusion Science and Technology
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Glass strategy: Hanford’s enhanced waste glass program
The mission of the Department of Energy’s Office of River Protection (ORP) is to complete the safe cleanup of waste resulting from decades of nuclear weapons development. One of the most technologically challenging responsibilities is the safe disposition of approximately 56 million gallons of radioactive waste historically stored in 177 tanks at the Hanford Site in Washington state.
ORP has a clear incentive to reduce the overall mission duration and cost. One pathway is to develop and deploy innovative technical solutions that can advance baseline flow sheets toward higher efficiency operations while reducing identified risks without compromising safety. Vitrification is the baseline process that will convert both high-level and low-level radioactive waste at Hanford into a stable glass waste form for long-term storage and disposal.
Although vitrification is a mature technology, there are key areas where technology can further reduce operational risks, advance baseline processes to maximize waste throughput, and provide the underpinning to enhance operational flexibility; all steps in reducing mission duration and cost.
J. E. Klein
Fusion Science and Technology | Volume 67 | Number 2 | March 2015 | Pages 416-419
Proceedings of TRITIUM 2013 | doi.org/10.13182/FST14-T42
Articles are hosted by Taylor and Francis Online.
The reduction in hydride absorption rate due to ”blanketing” can be explained in terms of a reduced hydrogen partial pressure in the bed due to the accumulation of inerts (i.e. non-hydrogen isotopes) in the bed void volume. Literature results show reduced absorption rates when protium for bed absorption contains helium with low-end inert compositions in the 0.6 to 1% range. A hydride bed containing 9.66 kg of LaNi4.25Al0.75 (LANA0.75) metal hydride - a nominal capacity of 1400 STP-L, was cycled repeatedly to decrepitate the hydride material into smaller particles for bed strain measurement. The hydride cycles added and removed nominally 1000 to 1100 STP-L of protium per hydride cycle. Consistent and repeatable absorptions results were observed for different absorption cycles. During one of the absorption tests, slower absorption results were obtained due to the use of typical grade (500 ppm inerts), instead of research grade, protium which blanketed the bed. The impact of 0.05% inerts in protium on bed absorption rate is shown and explained in terms of an increase in inert partial pressure as the bed was loaded.