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Glass strategy: Hanford’s enhanced waste glass program
The mission of the Department of Energy’s Office of River Protection (ORP) is to complete the safe cleanup of waste resulting from decades of nuclear weapons development. One of the most technologically challenging responsibilities is the safe disposition of approximately 56 million gallons of radioactive waste historically stored in 177 tanks at the Hanford Site in Washington state.
ORP has a clear incentive to reduce the overall mission duration and cost. One pathway is to develop and deploy innovative technical solutions that can advance baseline flow sheets toward higher efficiency operations while reducing identified risks without compromising safety. Vitrification is the baseline process that will convert both high-level and low-level radioactive waste at Hanford into a stable glass waste form for long-term storage and disposal.
Although vitrification is a mature technology, there are key areas where technology can further reduce operational risks, advance baseline processes to maximize waste throughput, and provide the underpinning to enhance operational flexibility; all steps in reducing mission duration and cost.
Yi-Hyun Park, In-Keun Yu, Mu-Young Ahn, Seungyon Cho, Duck Young Ku
Fusion Science and Technology | Volume 62 | Number 1 | July-August 2012 | Pages 185-189
Blanket Materials Technology | Proceedings of the Fifteenth International Conference on Fusion Reactor Materials, Part A: Fusion Technology | doi.org/10.13182/FST12-A14133
Articles are hosted by Taylor and Francis Online.
Lithium orthosilicate (Li4SiO4) pebbles are the primary candidate breeder for the Korean Helium-Cooled Solid Breeder test blanket module because of their superior overall performance qualities such as reasonable lithium atom density, favorable tritium release behavior, low activation property, and chemical stability. The aim of this study is to develop a fabrication method for Li4SiO4 pebbles with high sphericity and stable micro-crystalline structure. Li4SiO4 slurry was prepared by mixing Li4SiO4 powder and polyvinyl alcohol (PVA) solution. The Li4SiO4 gel-spheres were made by dropping slurry mixture into hydrogen peroxide (H2O2) solution. The gel-spheres were floated up to the surface of the H2O2 solution after staying at the bottom for a while and then aged on the surface of the H2O2 solution. The gel-spheres were dried at room temperature and sintered at several temperatures for 4 hours in air atmosphere. The sintered pebbles kept the shape of spheres during the sintering process in spite of shrinkage. Furthermore, the pebbles had relatively high sphericity. Also, the effects of PVA content and sintering temperature on the properties of the Li4SiO4 pebbles were investigated.