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Researchers report fastest purification of astatine-211 needed for targeted cancer therapy
Astatine-211 recovery from bismuth metal using a chromatography system. Unlike bismuth, astatine-211 forms chemical bonds with ketones.
In a recent study, Texas A&M University researchers have described a new process to purify astatine-211, a promising radioactive isotope for targeted cancer treatment. Unlike other elaborate purification methods, their technique can extract astatine-211 from bismuth in minutes rather than hours, which can greatly reduce the time between production and delivery to the patient.
“Astatine-211 is currently under evaluation as a cancer therapeutic in clinical trials. But the problem is that the supply chain for this element is very limited because only a few places worldwide can make it,” said Jonathan Burns, research scientist in the Texas A&M Engineering Experiment Station’s Nuclear Engineering and Science Center. “Texas A&M University is one of a handful of places in the world that can make astatine-211, and we have delineated a rapid astatine-211 separation process that increases the usable quantity of this isotope for research and therapeutic purposes.”
The researchers added that this separation method will bring Texas A&M one step closer to being able to provide astatine-211 for distribution through the Department of Energy’s Isotope Program’s National Isotope Development Center as part of the University Isotope Network.
Details on the chemical reaction to purify astatine-211 are in the journal Separation and Purification Technology.
N. G. Borisenko, I. V. Akimova, A. I. Gromov, A. M. Khalenkov, Yu. A. Merkuliev, V. N. Kondrashov, J. Limpouch, J. Kuba, E. Krousky, K. Masek, W. Nazarov, V. G. Pimenov
Fusion Science and Technology | Volume 49 | Number 4 | May 2006 | Pages 676-685
Technical Paper | Target Fabrication | dx.doi.org/10.13182/FST06-A1185
Articles are hosted by Taylor and Francis Online.
Fabrication methods for low-density fine-structure (cell size < 1 m) 3-D networks of cellulose triacetate (TAC) are developed. Target densities ranged 4-20 mg/cm3, similar polymer structures were produced both with no load and with high-Z cluster dopant with concentration up to 30%. Foams of varying density down to 0.25 plasma critical density at the third harmonic of iodine laser wavelength are supplied for laser shots. Closed-cell and 3-D network structures are considered and monitored as the means of thermal and radiation control in plasma. In comparative foam-and-foil laser irradiation experiments on PALS (Czech, Prague) laser facility the presently developed TAC targets were used along with earlier reported TMPTA (trimethylol propane triacrilate) and agar foams. Radiation transport and hydrodynamic wave velocities proved to be similar in TAC and TMPTA volume structures both having the form of regular 3-D networks, but differed a lot when TAC was compared to agar foams. Radiation transport during laser pulse in TAC doped with Cu-clusters was faster then in TAC with no dopant, whereas plasma from TAC doped with Cu-clusters cooled down quicker then with no clusters. High-Z cluster dopant is effective tool to control energy transport in underdense plasma.