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INL reports findings on unusual quantum behavior of plutonium
Scientists at Idaho National Laboratory have discovered that plutonium hexaboride (PuB6) displays a type of unusual quantum property called a topological Kondo insulating state. Materials with this property are neither typical electricity conductors nor regular insulators. Rather, they have exterior surfaces that strongly conduct electricity and interiors that block electricity.
Ken Nakajima, Masanori Akai
Nuclear Technology | Volume 113 | Number 3 | March 1996 | Pages 375-379
Technical Note | Fission Reactor | doi.org/10.13182/NT96-A35217
Articles are hosted by Taylor and Francis Online.
To investigate the accuracy of the neutronic calculations in various neutron spectra, the modified conversion ratios [(MCR): ratio of 238U capture rate-to-total fission rate] of four kinds of light water-moderated UO2 fuel lattices were measured. In the measurements, the relative reaction rates of 238U capture and total fission were obtained from the nondestructive gamma-ray spectrometry of 239Np and 143 Ce, respectively, which accumulated in the fuel rod irradiated at the Tank-Type Critical Assembly. The moderator-to-fuel volume ratios Vm/Vf of the measured lattices were 1.50 (undermoderate) to 3.00 (overmoderate). The measured MCRs were 0.477 ± 0.014(Vm/Vf = 1.50), 0.434 ± 0.013(1.83), 0.383 ± 0.011(2.48), and 0.356 ± 0.011(3.00), respectively. The Monte Carlo calculation employing the JENDL-3 library showed good agreement with the experiments for all the cores, although they showed a tendency of overestimation for larger values of MCR, as shown in the case of UO2 tight lattices. Therefore, it was concluded that, for the cores investigated, the accuracy of the neutronic calculation method currently used was very good.