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INL reports findings on unusual quantum behavior of plutonium
Scientists at Idaho National Laboratory have discovered that plutonium hexaboride (PuB6) displays a type of unusual quantum property called a topological Kondo insulating state. Materials with this property are neither typical electricity conductors nor regular insulators. Rather, they have exterior surfaces that strongly conduct electricity and interiors that block electricity.
M. E. Dunn, B. Basoglu, C. L. Bentley, C. Haught, M. J. Plaster, A. D. Wilkinson, T. Yamamoto, H. L. Dodds
Nuclear Technology | Volume 111 | Number 2 | August 1995 | Pages 183-196
Technical Paper | Nuclear Criticality Safety Special / Fission Reactor | doi.org/10.13182/NT95-A35129
Articles are hosted by Taylor and Francis Online.
The multigroup Monte Carlo code KENO V.a and the 238- and 44-energy-group ENDF/B-V cross-section libraries were validated for 233U systems. Fifty-one critical experiments involving 233UO2(NO3)2, 233UO2F2, or 233U metal were selected for the validation. The H/233U ratios for the experiments range from 0 to 1986. Each experiment was modeled with KENO V.a, and the effective multiplication factor keff was calculated for each system using the 44- and 238-group ENDF/B-V, the 27- and 218-group ENDF/B-IV, and the 16-group Hansen-Roach cross-section libraries. The mean calculated keff for all experiments using the 44- and 238-group libraries is 1.0090 ± 0.0021 and 1.0064 ± 0.0020, respectively. For comparison, the mean calculated keff using the 27-, 218-, and 16-group libraries is 1.0142 ± 0.0038, 1.0125 ± 0.0038, and 0.9991 ± 0.0019, respectively. In general, an improvement exists in the agreement between the calculated keff’s and the experimental results (i.e., keff= 1.0) obtained with the newer ENDF/B-V libraries relative to ENDF/B-IV.