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INL reports findings on unusual quantum behavior of plutonium
Scientists at Idaho National Laboratory have discovered that plutonium hexaboride (PuB6) displays a type of unusual quantum property called a topological Kondo insulating state. Materials with this property are neither typical electricity conductors nor regular insulators. Rather, they have exterior surfaces that strongly conduct electricity and interiors that block electricity.
Daniel Magallon, Hermann Hohmann, Hubert Schins
Nuclear Technology | Volume 98 | Number 1 | April 1992 | Pages 79-90
Technical Paper | Fast Reactor Safety / Nuclear Reactor Safety | doi.org/10.13182/NT92-A34652
Articles are hosted by Taylor and Francis Online.
Two experiments known as Tl and T2 are performed in the test section TERMOS of the FARO facility. Quantities of the order of 100 kg of molten pure UO2 ∼3000°C are poured into 130 kg of sodium at 400°C and 0.1 MPa contained in a 0.28-m-diam test tube over a height of 2.5 m. The tests show a melt delivery rate twice as high in T2 as in Tl. Because of the large scale of the experiment, the tests reveal new features concerning this type of interaction. Particularly, fuel/coolant interaction (FCI) occurs that induces stepwise penetration and dispersion of the melt, and a limitation of the melt quantity that could penetrate into the sodium. Sodium pressure peaks up to 6.0 MPa and pressurizations of the 0.150-m3 gas phase blanket up to 0.8 MPa are recorded. These FCIs are interpreted as vapor explosions in nearly saturated sodium. Quantities of 60 kg for Tl and 45 kg for T2 of UO2 fragments are collected in the debris catcher located at the bottom of the test tube. A debris bed structure resulting from this type of interaction is identified and characterized. Porosity is almost constant all over the bed height while permeability increases by a factor of 30 when going from the top to the bottom of the bed.