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The Standards Committee is responsible for the development and maintenance of voluntary consensus standards that address the design, analysis, and operation of components, systems, and facilities related to the application of nuclear science and technology. Find out What’s New, check out the Standards Store, or Get Involved today!
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Strontium: Supply-and-demand success for the DOE’s Isotope Program
The Department of Energy’s Isotope Program (DOE IP) announced last week that it would end its “active standby” capability for strontium-82 production about two decades after beginning production of the isotope for cardiac diagnostic imaging. The DOE IP is celebrating commercialization of the Sr-82 supply chain as “a success story for both industry and the DOE IP.” Now that the Sr-82 market is commercially viable, the DOE IP and its National Isotope Development Center can “reassign those dedicated radioisotope production capacities to other mission needs”—including Sr-89.
M. Grosse
Nuclear Technology | Volume 170 | Number 1 | April 2010 | Pages 272-279
Technical Paper | Special Issue on the 2008 International Congress on Advances in Nuclear Power Plants / Materials for Nuclear Systems | doi.org/10.13182/NT10-A9464
Articles are hosted by Taylor and Francis Online.
Isothermal and transient steam oxidation kinetics of the fuel rod cladding materials Duplex, M5™, E110, and Zircaloy-4 (Zry-4) were determined in separate-effect tests at various temperatures between 1073 and 1673K. All materials show parabolic time dependence at all temperatures, at least at the beginning of the oxidation. The temperature dependence of the oxidation rate is Arrhenius-like. All materials investigated show changes in the activation energy of the steam oxidation connected with the tetragonal-monoclinic phase transformation in the oxide. The temperatures of these changes differ between the Zr-Sn (Zry-4, Duplex: 1223 to 1273 K) and the Zr-Nb alloys (M5™, E110: 1273 to 1323 K). At temperatures below this phase transition, parts of the oxide layer can spall after longer oxidation times. It is known as the so-called "breakaway effect." This effect occurs in Zry-4 and E110, whereas it was not detected in Duplex and M5™. The breakaway effect results in nearly linear oxidation kinetics. The width of the temperature range and the morphology of the spalled oxide parts differ significantly between Zry-4 and E110. For Zry-4, the breakaway effect was found only at temperatures between 1233 and 1313 K. The spalling of the oxide layer at E110 was detected between 1073 and 1313 K. This wide temperature range also affects the transient steam oxidation behavior. For heating rates below 0.1 K/s, a stronger oxidation was found than expected for parabolic oxidation behavior. The oxide parts spalled from E110 specimens are much finer than the particles after breakaway from Zry-4.