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Reimagining nuclear materials for the future of medicine
Nuclear medicine has come a long way since Henri Becquerel first observed the penetrating energy of radioactive materials in 1896. Today, technetium-99m alone is used in more than 40 million diagnostic procedures every year—from cardiovascular imaging and bone scans to cancer detection—making it the undisputed workhorse of nuclear medicine. That single statistic tells you something important: An enormous portion of modern diagnostic medicine rests on a surprisingly narrow foundation, one built around a small number of aging research reactors that were never originally designed for continuous isotope production.
Rachel A. Shapiro, Massimiliano Fratoni
Nuclear Technology | Volume 194 | Number 1 | April 2016 | Pages 15-27
Technical Paper | doi.org/10.13182/NT15-97
Articles are hosted by Taylor and Francis Online.
Fully ceramic microencapsulated (FCM) fuel consists of TRISO (tristructural-isotropic) fuel particles embedded in a ceramic matrix (SiC) to form fuel pellets and rods and offers improved fission product retention and lower operating temperature with expected superior performance in normal and off-normal conditions compared to conventional fuel. When coupled with SiC cladding, FCM fuel eliminates zirconium altogether and is expected to drastically reduce hydrogen generation during a beyond-design-basis accident. In order to be deployed in current or future pressurized water reactors (PWRs), FCM fuel must meet or exceed the neutronic performance of conventional fuel. Limited by low heavy metal loading, an FCM fuel assembly requires increased enrichment and large fuel rods to match the cycle length of a conventional fuel assembly.
This study investigated the core design, neutronics, and thermal hydraulics of a PWR loaded with FCM fuel and sought to optimize the assembly design to minimize the enrichment required to reach fuel performance similar to that of conventional fuel. It was found that the implementation of FCM fuel in a 17 × 17 assembly requires close to 20% enrichment and large fuel rods. Such design performs comparably to conventional fuel (4.5% enrichment) in terms of cycle length, reactivity coefficients, intra-assembly power peaking factor, burnable poison penalty, and control rod worth but requires an increase of pumping power. A parametric analysis spanned a large design space varying fuel outer diameter and pitch-to-diameter ratio (P/D) and downselected two alternate assembly designs: 11 × 11 (1.65-cm outer diameter and 1.18 P/D) and 9 × 9 (2.12-cm outer diameter and 1.12 P/D). These designs meet the cycle length requirement with 18.6% and 16.2% enrichments, respectively, but feature a smaller minimum departure from nucleate boiling ratio (MDNBR) compared to a reference assembly. It was estimated that a slight increase in rod outer diameter increases MDNBR to the desired level and implies a pressure drop increase of 10%.
