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Undeclared uranium hitches a ride on cobalt exports from Congo, study says
Philippe (left) and Manzuk quantified the amount of uranium that has been exported from the DRC in cobalt shipments or left behind in the environment. (Photo: Joel Hallberg/UW–Madison)
Researchers at the University of Wisconsin–Madison and Princeton University have published a study in Nature Communications that calls attention to a blind spot in nuclear nonproliferation: The Democratic Republic of the Congo (DRC) has exported thousands of metric tons of uranium, and there is no accounting for where it has gone.
In partnership with Lighthouse Reports and the Financial Times, UW–Madison nuclear engineering professor and nuclear security expert Sébastien Philippe and Ryan Manzuk, a geologist and research fellow in Philippe’s group and at Princeton, conducted the study using countrywide mineralization and geochemical data.
K. S. Smith, T. Bahadir, R. Ferrer, D. B. Lancaster, A. J. Machiels
Nuclear Technology | Volume 185 | Number 1 | January 2014 | Pages 39-56
Technical Paper | Fuel Cycle and Management | doi.org/10.13182/NT13-31
Articles are hosted by Taylor and Francis Online.
Pressurized water reactor (PWR) assembly reactivity distributions are inferred from ∼600 in-core flux maps taken during 44 cycles of operation of the Catawba and McGuire nuclear power plants. The reactivity distribution for each flux map is determined by systematically searching for fuel subbatch reactivities that minimize differences between measured and computed 235U fission rates. More than eight million core calculations are used to reduce one million measured signals to a set of ∼2500 experimental fuel reactivities for fuel with up to 55 GWd/T burnup. These measured reactivity changes with depletion can be used to validate computer code systems used for burnup credit. To reduce the effort required to quantify computer code system biases and uncertainties, the measured changes in fuel depletion reactivity have been reduced to a set of experimental PWR lattice benchmarks for the change in reactivity as a function of fuel burnup. Results demonstrate that the uncertainty of hot-full-power (HFP) depletion reactivity of the benchmarks is < 250 pcm up to 55 GWd/T burnup. Oak Ridge National Laboratory's TSUNAMI tools are used to extend HFP results to cold conditions, and reactivity decrement uncertainties increase to ∼600 pcm. These experimental benchmarks provide a basis for quantification of combined nuclide inventory and cross-section uncertainties in computed reactivity decrements. It is demonstrated that flux map data reduction is not sensitive to the analytical tools (CASMO/SIMULATE) employed here, and experimental fuel depletion reactivity decrements and uncertainties are anticipated to be independent of fuel management code system use for the data reduction. For CASMO-based analysis, the HFP reactivity burnup decrement biases are shown to be <250 pcm up to 55 GWd/T burnup, and results show that the historical “Kopp memo” 5% reactivity decrement uncertainty assumption is conservative.