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Glass strategy: Hanford’s enhanced waste glass program
The mission of the Department of Energy’s Office of River Protection (ORP) is to complete the safe cleanup of waste resulting from decades of nuclear weapons development. One of the most technologically challenging responsibilities is the safe disposition of approximately 56 million gallons of radioactive waste historically stored in 177 tanks at the Hanford Site in Washington state.
ORP has a clear incentive to reduce the overall mission duration and cost. One pathway is to develop and deploy innovative technical solutions that can advance baseline flow sheets toward higher efficiency operations while reducing identified risks without compromising safety. Vitrification is the baseline process that will convert both high-level and low-level radioactive waste at Hanford into a stable glass waste form for long-term storage and disposal.
Although vitrification is a mature technology, there are key areas where technology can further reduce operational risks, advance baseline processes to maximize waste throughput, and provide the underpinning to enhance operational flexibility; all steps in reducing mission duration and cost.
Kenneth Hoar, Piotr Nowinski, Vernon Hodge, James Cizdziel
Nuclear Technology | Volume 175 | Number 1 | July 2011 | Pages 351-359
Technical Paper | Special Issue on the 16th Biennial Topical Meeting of the Radiation Protection and Shielding Division / Environmental Effects of Nuclear Technology | doi.org/10.13182/NT11-A12307
Articles are hosted by Taylor and Francis Online.
Rock varnish samples were collected near three point sources of air pollution to determine if the varnish contained a record of recent air pollution. Samples were collected as follows: downwind of the Nevada Test Site (NTS); in the fallout pattern of the shuttered Mohave Power Plant, located in Laughlin, Nevada; and, near the operating Reid-Gardner Power Plant, just east of Las Vegas, Nevada. Analysis of the NTS rock varnish shows 240Pu/239Pu mass ratios as low as 0.0592 ± 0.0003 and 241Pu/239Pu ratios as low as 0.00063 ± 0.00004, compared to worldwide values of 0.18 ± 0.01 and 0.009 ± 0.002, respectively, clearly indicating that the varnish can be used as a forensic tool for identifying the source of air pollution, in this case the NTS. The samples collected in the plumes of the coal-fired power plants contain thorium and uranium, and have 232Th/238U mass ratios from 1 to 30, and concentrations from 5 to 755 ppm for Th and 1 to 578 ppm for U. The highest concentrations of these elements occur together at locations that implicate the power plants; however, additional samples would be required to demonstrate unequivocally that the power plants are the sources. Overall, it is apparent that rock varnish can be utilized as a passive monitor to investigate recent air pollution.