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GAO: Clarification of HLW definition could save DOE billions
A clearer definition of what constitutes high-level radioactive waste could save the Department of Energy’s Office of Environmental Management “tens of billions of dollars” in waste management costs and accelerate its cleanup schedule by decades, according to a report by the U.S. Government Accountability Office.
DOE-EM’s efforts to manage waste resulting from legacy spent nuclear fuel reprocessing have been hindered for decades by the ambiguity of the statutory definition of HLW as laid out in the Atomic Energy Act and Nuclear Waste Policy Act, the report states. While admitting that the DOE has taken steps to overcome this ambiguity, the GAO says that the department has not fully evaluated all available opportunities to treat and dispose of waste more economically as either transuranic or low-level radioactive waste.
James R. Allensworth, Michael F. Simpson, Man-Sung Yim, Supathorn Phongikaroon
Nuclear Technology | Volume 181 | Number 2 | February 2013 | Pages 337-348
Technical Paper | Reprocessing | doi.org/10.13182/NT13-A15788
Articles are hosted by Taylor and Francis Online.
Methods to improve fission product salt sorption into zeolite-A have been investigated in an effort to reduce waste associated with the electrochemical treatment of spent nuclear fuel. It was demonstrated that individual fission product chloride salts were absorbed by zeolite-A in a solid-state process. As a result, recycling of LiCl-KCl appears feasible via adding a zone-freezing technique to the current treatment process. Ternary salt molten-state experiments showed the limiting kinetics of CsCl and SrCl2 sorption into the zeolite. CsCl sorption occurred rapidly relative to SrCl2 with no observed dependence on zeolite particle size, while SrCl2 sorption was highly dependent on particle size. The application of experimental data to a developed reaction-diffusion-based sorption model yielded diffusivities of 8.04 × 10-6 and 4.04 × 10-7 cm2 /s for CsCl and SrCl2, respectively. Additionally, the chemical reaction term in the developed model was found to be insignificant compared to the diffusion term.
