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Glass strategy: Hanford’s enhanced waste glass program
The mission of the Department of Energy’s Office of River Protection (ORP) is to complete the safe cleanup of waste resulting from decades of nuclear weapons development. One of the most technologically challenging responsibilities is the safe disposition of approximately 56 million gallons of radioactive waste historically stored in 177 tanks at the Hanford Site in Washington state.
ORP has a clear incentive to reduce the overall mission duration and cost. One pathway is to develop and deploy innovative technical solutions that can advance baseline flow sheets toward higher efficiency operations while reducing identified risks without compromising safety. Vitrification is the baseline process that will convert both high-level and low-level radioactive waste at Hanford into a stable glass waste form for long-term storage and disposal.
Although vitrification is a mature technology, there are key areas where technology can further reduce operational risks, advance baseline processes to maximize waste throughput, and provide the underpinning to enhance operational flexibility; all steps in reducing mission duration and cost.
Indrajeet Singh, S. B. Degweker, Anurag Gupta
Nuclear Science and Engineering | Volume 189 | Number 2 | February 2018 | Pages 101-119
Technical Paper | doi.org/10.1080/00295639.2017.1388092
Articles are hosted by Taylor and Francis Online.
The fuel in high-temperature reactors (HTRs) is made up of tiny fuel particles (called TRISO particles) dispersed randomly in a graphite matrix. For the commonly used fuels, namely, enriched uranium or low-enriched uranium/233U mixed with Th, this dispersion may be treated as a homogeneous mixture at almost all neutron energies except at the resonances of the major nuclide (238U or 232Th) where the macroscopic cross section is so large that the neutron mean free path is comparable to the fuel kernel radius. In the equivalence theory approach used in many codes based on the WIMS-D library, this heterogeneity is accounted for by the escape cross section from a fuel kernel together with a carefully evaluated Dancoff correction factor.
In HTRs designed to burn plutonium, the fuel kernel contains oxides of various isotopes of Pu, and there is no fertile nuclide. Hence, the macroscopic cross section of the fuel is rather high in the thermal region, i.e., below 4 eV in the WIMS-D library (which also includes the two major resonances of 240Pu and 239Pu). For such fuels, the treatment of neutron transport in the thermal energy range must also include the random heterogeneous distribution of fuel in the graphite matrix. Since the resonance treatment method in the WIMS-D library, described above, is neither available nor applicable for thermal energies, a different method is clearly necessary.
HTR lattice codes such as WIMS and DRAGON use approximate collision probabilities between the various microscopic regions, namely, the fuel kernel, the coating layers, and the graphite matrix in the solution of the multigroup transport equation to account for this heterogeneity. In an earlier paper, we developed a simple though heuristic approach for solving this problem. In the present paper, we develop a more systematic theoretical method for solving the transport equation in a random dispersion by an exact evaluation of the collision probabilities in various regions of the lattice cell. The method has been incorporated in the collision probability code BOXER3. Comparison with benchmarks of Pu-based HTR fuels shows very good agreement thus validating the new approach. The method is likely to have application beyond the problem discussed in the paper.