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Glass strategy: Hanford’s enhanced waste glass program
The mission of the Department of Energy’s Office of River Protection (ORP) is to complete the safe cleanup of waste resulting from decades of nuclear weapons development. One of the most technologically challenging responsibilities is the safe disposition of approximately 56 million gallons of radioactive waste historically stored in 177 tanks at the Hanford Site in Washington state.
ORP has a clear incentive to reduce the overall mission duration and cost. One pathway is to develop and deploy innovative technical solutions that can advance baseline flow sheets toward higher efficiency operations while reducing identified risks without compromising safety. Vitrification is the baseline process that will convert both high-level and low-level radioactive waste at Hanford into a stable glass waste form for long-term storage and disposal.
Although vitrification is a mature technology, there are key areas where technology can further reduce operational risks, advance baseline processes to maximize waste throughput, and provide the underpinning to enhance operational flexibility; all steps in reducing mission duration and cost.
Dan G. Cacuci
Nuclear Science and Engineering | Volume 183 | Number 1 | May 2016 | Pages 1-21
Technical Paper | doi.org/10.13182/NSE15-81
Articles are hosted by Taylor and Francis Online.
This work presents an illustrative application of the second-order adjoint sensitivity analysis methodology (2nd-ASAM) to a heat transport benchmark problem that simulates the radial heat conduction in a heated fuel rod together with the axial heat transport along the coolant channel surrounding the rod. This paradigm benchmark is sufficiently simple to admit an exact solution, thereby making transparent the mathematical derivations underlying the 2nd-ASAM, and also for performing solution verification of computational fluid dynamics simulation tools such as the FLUENT Adjoint Solver, a code that has been used for computing thermal-hydraulic processes within the G4M Reactor. The G4M Reactor is an innovative small modular fast reactor cooled by lead-bismuth eutectic.
The benchmark problem has six thermal-hydraulic parameters representative of the G4M Reactor, as well as of a test section that is under design for analyzing thermal-hydraulic phenomena expected within the reactor’s core. Thus, the benchmark exhibits 6 first-order and 21 second-order sensitivities for the temperature distribution at any location within the heated rod (and/or on its surface) and just as many sensitivities for the temperature distribution at any location within the coolant. Locations of particular importance are those where the rod temperature attains its maximum along the rod’s axis or on the rod’s surface, as well as the coolant’s exit, where the coolant temperature attains its maximum.
The general theory underlying the 2nd-ASAM indicates that for a physical system comprising Nα parameters, the computation of all of the first- and second-order response sensitivities requires Nα large-scale computations involving correspondingly constructed adjoint systems, which we called second-level adjoint sensitivity systems (2nd-LASS). In practice, however, the actual number of large-scale adjoint computations can be significantly smaller; in particular, all 54 first- and second-order rod and coolant temperature sensitivities for the benchmark presented in this work were obtained using only seven independent adjoint computations. Furthermore, the construction and solution of the 2nd-LASS require very little additional effort beyond the construction of the first-level adjoint sensitivity system (1st-LASS) needed for computing the first-order sensitivities. Very significantly, only the sources on the right side of the differential operator needed to be modified; the left side of the respective differential equations (and hence the solver in large-scale practical applications) remained unchanged from the 1st-LASS and from the original equations when these are linear in the unknown state function.
This work also shows that the second-order sensitivities have the following impacts on the computed moments of the response distribution: (a) they cause the expected value of the response to differ from the computed nominal value of the response, (b) they contribute to the response variances and covariances, and (c) they contribute decisively to causing asymmetries in the response distribution. Indeed, neglecting the second-order sensitivities would nullify the third-order response correlations stemming from normally distributed parameters and hence would nullify the skewness of the response; consequently, events occurring in a response’s long and/or short tails could be missed.