Design of a Subcritical Assembly for Conducting Neutron Activation Analyses in the Field

Two subcritical assemblies (consisting of a subcritical reactor plus a neutron emitter such as ²⁵²Cf) designed for conducting neutron activation analyses in the field are described. The size of the assemblies has been minimized (compared to conventional, graphite-moderated assemblies) to allow for field portability. Although less powerful than using a research reactor as the source of neutrons, these assemblies will provide an adequate source of neutrons for detecting gold concentrations in rock or soil samples down to the limits of economic importance. Using a field-portable source of neutrons eliminates the need for shipping samples back to the reactor for analysis, which may be important for reasons of sample security and measurement turnaround time. The two subcritical assemblies are composed of natural uranium metal as the multiplying material and high-density polyethylene as the moderator, and they have k_eff approximately equal to 0.8 for the smaller assembly (~692-kg assembly mass) and 0.9 for the larger assembly (~3059-kg assembly mass). The larger assembly was found to be more desirable from a neutronics standpoint; however, it may be too massive to maintain field portability. It was found that the optimal location for the irradiation facility (a 4.0-cm-high, 2.0-cm-diam right cylinder) in the subcritical assemblies is the grid location as close to the neutron emitter location as possible. It was also found that the total, epithermal plus thermal (i.e., neutron energy <0.5 eV), and thermal (i.e., neutron energy <0.05 eV) volume-averaged neutron fluxes were as follows (assuming a neutron emitter source strength of 10⁹ n/s): 1.72 × 10⁸, 4.47 × 10⁷, and 2.15 × 10⁷ cm^-2s^-1 for the smaller assembly, and 3.43 × 10⁸, 9.09 × 10⁷, and 4.37 × 10⁷ cm^-2s^-1 for the larger assembly. Although the purpose for which the assembly was designed was for conducting neutron activation analyses for gold, the assemblies should also work equally well for analyzing sample compositions of other elements at both the bulk and trace levels.