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Fusion Science and Technology
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Glass strategy: Hanford’s enhanced waste glass program
The mission of the Department of Energy’s Office of River Protection (ORP) is to complete the safe cleanup of waste resulting from decades of nuclear weapons development. One of the most technologically challenging responsibilities is the safe disposition of approximately 56 million gallons of radioactive waste historically stored in 177 tanks at the Hanford Site in Washington state.
ORP has a clear incentive to reduce the overall mission duration and cost. One pathway is to develop and deploy innovative technical solutions that can advance baseline flow sheets toward higher efficiency operations while reducing identified risks without compromising safety. Vitrification is the baseline process that will convert both high-level and low-level radioactive waste at Hanford into a stable glass waste form for long-term storage and disposal.
Although vitrification is a mature technology, there are key areas where technology can further reduce operational risks, advance baseline processes to maximize waste throughput, and provide the underpinning to enhance operational flexibility; all steps in reducing mission duration and cost.
L. A. Sedano
Fusion Science and Technology | Volume 48 | Number 1 | July-August 2005 | Pages 605-608
Technical Paper | Tritium Science and Technology - Materials Interaction and Permeation | doi.org/10.13182/FST05-A998
Articles are hosted by Taylor and Francis Online.
The H (or D, or T) Sievert's constant for liquid Sn-Li alloys is calculated from thermodynamic data issuing of the Sn-Li binary phase diagram analysis. The range of temperatures investigated is 600-873 K (Sn0.8Li0.2 m.p. ~ 599 K) to maintain single-phase binary melts. The thermodynamic functions of Li-H, Sn-H, Sn-Li are evaluated to derive those of Sn-Li-H. Thus, monotectic solubility data for Sn and Li is analyzed. The calculation is done for high-dilution conditions. A quasi-chemical regular solution model is used for temperature/composition extrapolations when no data is available. The tritium Sievert's constant in Sn0.8Li0.2 at 600 K is: 9.65 10-8 Pa-12, five times the Reiter's measured value for Pb-17Li and ~ 6 times the value in Pb-17Li eutectic obtained by using the same theoretical approach.