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Fusion Science and Technology
Latest News
Glass strategy: Hanford’s enhanced waste glass program
The mission of the Department of Energy’s Office of River Protection (ORP) is to complete the safe cleanup of waste resulting from decades of nuclear weapons development. One of the most technologically challenging responsibilities is the safe disposition of approximately 56 million gallons of radioactive waste historically stored in 177 tanks at the Hanford Site in Washington state.
ORP has a clear incentive to reduce the overall mission duration and cost. One pathway is to develop and deploy innovative technical solutions that can advance baseline flow sheets toward higher efficiency operations while reducing identified risks without compromising safety. Vitrification is the baseline process that will convert both high-level and low-level radioactive waste at Hanford into a stable glass waste form for long-term storage and disposal.
Although vitrification is a mature technology, there are key areas where technology can further reduce operational risks, advance baseline processes to maximize waste throughput, and provide the underpinning to enhance operational flexibility; all steps in reducing mission duration and cost.
Masahiko Utsuro, Mitsuo Nakai, Hideki Kohri, Takeshi Ohta, Takumi Konno, Asako Igashira, Mamoru Fujiwara
Fusion Science and Technology | Volume 78 | Number 7 | October 2022 | Pages 513-527
Technical Paper | doi.org/10.1080/15361055.2022.2062098
Articles are hosted by Taylor and Francis Online.
A test experiment to polarize tritium nuclei to develop a polarized deuterium-tritium (D-T) laser fusion concept is proposed in which a ferromagnetic complex with a high internal magnetic field is used to polarize tritium nuclei on physisorbed D-T molecules with an internal β-decay heat load in a D-T target. Heteronuclear hydrogen deuteride (HD) is used to conduct the measurements herein instead of as in typical D-T–based experiments. As proof-of-concept experimentation, the adsorption and desorption characteristics of HD are examined on Prussian blue ferromagnetic analogue Ni3[Fe(CN)6]2 at temperatures of 77 K and around 23 K. Nuclear magnetic resonance (NMR) analysis of the ferromagnetic complex-mediated adsorption of HD onto activated carbon pellets at 10 K is conducted step by step using a multilocular probe cell that had been simplified to give a single-tube probe cell. The resulting 1H NMR spectra are compared with 19F NMR spectra obtained for reference on a Kel-F probe cell wall. Slight differences between the calculated NMR frequency from the gyromagnetic ratio and the actually observed NMR frequency are also discussed.