Purdue team uses Argonne’s APS for 3D view of irradiated fuelNuclear NewsResearch & ApplicationsJanuary 22, 2021, 9:32AM|Nuclear News StaffImage: Purdue University/Maria OkuniewskiA team of researchers led by Purdue University has used X-ray imaging conducted at Argonne National Laboratory’s Advanced Photon Source to obtain a three-dimensional view of the interior of an irradiated nuclear fuel sample. The use of synchrotron micro-computed tomography could lead to more accurate modeling of fuel behavior and more efficient nuclear fuel designs, according to the researchers.The results of the study were published in the Journal of Nuclear Materials, in a paper titled “The application of synchrotron micro-computed tomography to characterize the three-dimensional microstructure in irradiated nuclear fuel,” and were also described in a press release issued by Argonne and Purdue University on January 19.Technique: Micro-computed tomography detects an X-ray beam as it emerges on the other side of the sample. From multiple images taken as a sample is rotated, the internal features of a sample can be imaged based on how the X-ray beam was altered as it passed through the sample.At Argonne, the Purdue research team worked with scientists at beamline 1-ID-E, a high-brilliance X-ray source at the APS, to examine the sample. The research marked the first time that synchrotron X-ray micro-computed tomography was used to analyze the morphology of the microstructure of irradiated nuclear fuel in three dimensions, according to the research team.The sample: The subject of investigation was a tiny piece of uranium-zirconium (U-10Zr) from a fuel pin that spent two years at full power in the Fast Flux Test Facility at the Hanford Site, near Richland, Wash., before it was extracted in the early 1990s.The sample was prepared at Idaho National Laboratory. A cube of the material about 100 microns across—about the width of a human hair—was milled from a fuel pin using a focused ion beam with scanning electron microscopy. “We had to wait decades for this fuel to radiologically cool, or decay,” said Maria Okuniewski, an assistant professor of materials engineering at Purdue University and the paper’s lead author. “It was literally the coolest specimen that we could remove, based on the permissible safety guidelines at both INL and APS.”Findings: Okuniewski and her colleagues wanted to characterize swelling caused by the accumulation of gaseous fission by-products, which limits the useful life of nuclear fuels.The study revealed the presence of pores and of three distinct uranium phase regions: poor, intermediate, and rich. The researchers determined that 7.2 percent of the fuel specimen was porous. Five growth stages of pore evolution were observed, including nucleation, growth, coalescence, interconnected porosity, and extended/interconnected porosity. The research also found that the release of fission gases might continue to occur beyond the thresholds assumed in previous analyses.“We’re always striving within the nuclear community to figure out ways that we can improve the fuel performance codes,” Okuniewski said. “This is one way to do that. Now we have three-dimensional insight that we previously didn’t have at all.”Tags:argonne national laboratorydoefuelidaho national laboratorymicro-computed tomographypurdue universityuranium-zirconium fuelShare:LinkedInTwitterFacebook
Fukiushima Daiichi: 10 years onThe Fukushima Daiichi site before the accident. All images are provided courtesy of TEPCO unless noted otherwise. It was a rather normal day back on March 11, 2011, at the Fukushima Daiichi nuclear plant before 2:45 p.m. That was the time when the Great Tohoku Earthquake struck, followed by a massive tsunami that caused three reactor meltdowns and forever changed the nuclear power industry in Japan and worldwide. Now, 10 years later, much has been learned and done to improve nuclear safety, and despite many challenges, significant progress is being made to decontaminate and defuel the extensively damaged Fukushima Daiichi reactor site. This is a summary of what happened, progress to date, current situation, and the outlook for the future there.Go to Article
Search for new Hanford tank waste contractor beginsWorkers retrieve waste from a single-shell tank at the Hanford Site earlier this year. Photo: DOEThe Department of Energy’s Office of Environmental Management (EM) has issued a draft request for proposals for the new Integrated Tank Disposition Contract at the Hanford Site near Richland, Wash. The 10-year, $26.5 billion contract will replace the Tank Operations Contract currently held by Washington River Protection Solutions, and the scope will be expanded to include the operation of the Waste Treatment and Immobilization Plant (WTP) after radiological, or “hot,” commissioning of the plant is completed.The DOE had awarded a tank closure contract to a team led by BWX Technologies in May of last year, but later rescinded that decision after protests were raised by the two losing contract bidders.About 56 million gallons of radioactive waste is contained in Hanford’s 177 aging underground tanks. The WTP, which is still under construction, will vitrify the waste after it has been separated into low- and high-activity waste streams.Go to Article
Researchers report fastest purification of astatine-211 needed for targeted cancer therapyAstatine-211 recovery from bismuth metal using a chromatography system. Unlike bismuth, astatine-211 forms chemical bonds with ketones.In a recent study, Texas A&M University researchers have described a new process to purify astatine-211, a promising radioactive isotope for targeted cancer treatment. Unlike other elaborate purification methods, their technique can extract astatine-211 from bismuth in minutes rather than hours, which can greatly reduce the time between production and delivery to the patient.“Astatine-211 is currently under evaluation as a cancer therapeutic in clinical trials. But the problem is that the supply chain for this element is very limited because only a few places worldwide can make it,” said Jonathan Burns, research scientist in the Texas A&M Engineering Experiment Station’s Nuclear Engineering and Science Center. “Texas A&M University is one of a handful of places in the world that can make astatine-211, and we have delineated a rapid astatine-211 separation process that increases the usable quantity of this isotope for research and therapeutic purposes.”The researchers added that this separation method will bring Texas A&M one step closer to being able to provide astatine-211 for distribution through the Department of Energy’s Isotope Program’s National Isotope Development Center as part of the University Isotope Network.Details on the chemical reaction to purify astatine-211 are in the journal Separation and Purification Technology.Go to Article
Demolition of former radioisotope lab underway at ORNLA view of the demolition of a hot cell inside a protective cover at the former radioisotope development lab at ORNL. Photo: DOEThe Department of Energy’s Oak Ridge Office of Environmental Management and contractor UCOR have begun removing the two remaining structures at the former radioisotope development laboratory at Oak Ridge National Laboratory, in Tennessee.“This project launches our next phase of major demolition and cleanup at ORNL,” said Nathan Felosi, ORNL’s portfolio federal project director for OREM. “Our work is eliminating contaminated structures, like this one, that are on DOE’s list of high-risk facilities and clearing space for future research missions.”The project is scheduled to be completed this spring, OREM reported on February 23.Go to Article
DOE steps up plutonium production for future space explorationThis high-resolution still image is from a video taken by several cameras as NASA’s Perseverance rover touched down on Mars on February 18. Credits: NASA/JPL-CaltechNASA’s Perseverance rover, which successfully landed on Mars on February 18, is powered in part by the first plutonium produced at Department of Energy laboratories in more than 30 years. The radioactive decay of Pu-238 provides heat to radioisotope thermoelectric generators (RTGs) like the one onboard Perseverance and would also be used by the Dynamic Radioisotope Power System, currently under development, which is expected to provide three times the power of RTGs.Idaho National Laboratory is scaling up the production of Pu-238 to help meet NASA’s production goal of 1.5 kg per year by 2026, the DOE announced on February 17.Go to Article
NASA’s radioisotope-powered science will persevere on MarsMembers of the Perseverance rover team in Mission Control at NASA’s Jet Propulsion Laboratory react after receiving confirmation of a successful landing. Photo: NASA/Bill IngallsNASA mission control and space science fans around the world celebrated the safe landing of the Mars 2020 Perseverance rover on February 18 after a journey of 203 days and 293 million miles. Landing on Mars is difficult—only about 50 percent of all previous Mars landing attempts have succeeded—and a successful landing for Perseverance, the fifth rover that NASA has sent to Mars, was not assured. Confirmation of the successful touchdown was announced at NASA’s Jet Propulsion Laboratory in Pasadena, Calif., at 3:55 p.m. EST.“This landing is one of those pivotal moments for NASA, the United States, and space exploration globally—when we know we are on the cusp of discovery and sharpening our pencils, so to speak, to rewrite the textbooks,” said acting NASA administrator Steve Jurczyk. “The Mars 2020 Perseverance mission embodies our nation’s spirit of persevering even in the most challenging of situations, inspiring, and advancing science and exploration. The mission itself personifies the human ideal of persevering toward the future and will help us prepare for human exploration of the Red Planet.”Only radioisotope thermoelectric generators (RTG) can provide the long-lasting, compact power source that Perseverance needs to carry out its long-term exploratory mission. Perseverance carries an RTG powered by the radioactive decay of plutonium-238 that was supplied by the Department of Energy. ANS president Mary Lou Dunzik-Gougar and CEO and executive director Craig Piercy congratulated NASA after the successful landing, acknowledging the critical contributions of the DOE’s Idaho National Laboratory, Oak Ridge National Laboratory, and Los Alamos National Laboratory.Go to Article
New Brunswick awards additional funding for SMR developmentNew Brunswick Premier Blaine Higgs announces C$20 million in funding for the ARC-100 small modular reactor. Photo: ARC CanadaThe Canadian province of New Brunswick has awarded C$20 million (about $15.7 million) to ARC Clean Energy Canada (ARC Canada) to support the development of the proposed ARC-100 advanced small modular reactor. The premier of New Brunswick, Blaine Higgs, announced the award during his state of the province address on February 10.ARC Canada, headquartered in Saint John, New Brunswick, is a subsidiary of U.S.-based ARC Clean Energy, formerly known as Advanced Reactor Concepts. The company’s ARC-100 is a 100-MWe integrated sodium-cooled fast reactor that uses a metallic uranium alloy fuel. Based on Argonne National Laboratory’s Experimental Breeder Reactor-II, the reactor is designed to operate for 20-plus years without refueling.In October 2019, ARC Canada announced that it had completed the first phase of the Canadian Nuclear Safety Commission’s (CNSC) vendor design review. (While the phase-one assessment provides detailed feedback regarding a vendor’s understanding of the CNSC’s requirements for a nuclear power plant in Canada, it does not certify the design or license the reactor.)Go to Article
INL seeks efficiency boost for radioisotope-powered spacecraftThe RTG used to power the Mars Perseverance rover is shown here being placed in a thermal vacuum chamber for testing in a simulated near-space environment. Source: INLThe Department of Energy’s Idaho National Laboratory is celebrating the scheduled landing of the Perseverance rover on the surface of Mars in just two days’ time with a live Q&A today, February 16, from 3 p.m. to 4:30 p.m. EST).INL and Battelle Energy Alliance, its management and operating contractor, are already looking ahead to the next generation of plutonium-powered spacecraft: the Dynamic Radioisotope Power System (Dynamic RPS). INL announced on February 15 that it is partnering with NASA and the DOE to seek industry engagement to further the design of this new power system.Go to Article
DOE extends comment period on VTR environmental reviewThe Department of Energy has extended the public review and comment period for the Draft Versatile Test Reactor Environmental Impact Statement (DOE/EIS-0542) through March 2, 2021.The DOE issued the draft EIS for the Versatile Test Reactor (VTR) for comment on December 21, 2020. The draft document identifies Idaho National Laboratory as the DOE’s preferred location for the VTR, a proposed sodium-cooled fast-neutron-spectrum test reactor that, according to the DOE, will enhance and accelerate research, development, and demonstration of innovative nuclear energy technologies.In August 2020, Battelle Energy Alliance, which operates INL for the DOE, began contract negotiations with a Bechtel National–led team that includes TerraPower and GE Hitachi Nuclear Energy to support the design and construction of the VTR.Go to Article
Savannah River crews remove cesium columns from tank closure unitWork crews remove the first column filled with cesium from the Tank Closure Cesium Removal unit by crane in H tank farm at the Savannah River Site. Photo: DOEColumns filled with cesium have been removed at the Savannah River Site in a demonstration project designed to accelerate removal of radioactive salt waste from underground tanks.“On the surface, it appeared to be like any other crane lift and equipment transport, which are routinely performed in the tank farms. However, this equipment contained cesium-rich, high-level waste, which was transported aboveground via roadway to an on-site interim safe storage pad,” said Savannah River Remediation (SRR) president and project manager Phil Breidenbach. “It was all handled safely and executed with outstanding teamwork by our highly skilled workforce.”Operated by liquid waste contractor SRR, a system known as the Tank Closure Cesium Removal (TCCR) unit removes cesium from the salt waste in Tank 10 in the site's H Tank Farm. The TCCR is a pilot demonstration that helps accelerate tank closure at the site, according to a report by the Department of Energy on February 9.Go to Article