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Reich-Moore Parameterization of ( ,n) Reactions on Light Nuclei: Impact on a Neutron Source Calculation in an Oxide Fuel

Volume 151 · Number 2 · October 2005 · Pages 135-156
Technical Paper

Richard Babut, Olivier Bouland, Eric Fort

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Evaluated data are adjusted on experimental measurements using nuclear reaction models. Among these data, those concerning alpha-particle interactions on light nuclei are not well known, although crucial for neutron emission problems via ( ,n) processes in nuclear fuels (oxide, carbide, nitride). Examples of applications are reprocessing, packaging and storage of radioactive waste, and intrinsic neutron source term evaluation in critical and subcritical reactors (accelerator-driven systems). The goal is the modeling of ( ,n) reactions on oxygen isotopes to extract the resonance parameters. The SAMMY code, which relies on the Reich-Moore approximation of the R-matrix theory, is used. In the most recent version, the SAMMY code allows the study of the in- and outgoing charged-particle channels. An important validation of this new feature has been made. In addition, a manifest lack of experimental data for this type of reaction has been underlined. Finally, the impact of the new pointwise description of the ( ,n) reaction cross section on the energy distribution calculation of the intrinsic neutron source of an irradiated mixed-oxide fuel pin is shown and compared to the standard calculation, which uses average cross sections.
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