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Glass strategy: Hanford’s enhanced waste glass program
The mission of the Department of Energy’s Office of River Protection (ORP) is to complete the safe cleanup of waste resulting from decades of nuclear weapons development. One of the most technologically challenging responsibilities is the safe disposition of approximately 56 million gallons of radioactive waste historically stored in 177 tanks at the Hanford Site in Washington state.
ORP has a clear incentive to reduce the overall mission duration and cost. One pathway is to develop and deploy innovative technical solutions that can advance baseline flow sheets toward higher efficiency operations while reducing identified risks without compromising safety. Vitrification is the baseline process that will convert both high-level and low-level radioactive waste at Hanford into a stable glass waste form for long-term storage and disposal.
Although vitrification is a mature technology, there are key areas where technology can further reduce operational risks, advance baseline processes to maximize waste throughput, and provide the underpinning to enhance operational flexibility; all steps in reducing mission duration and cost.
M. Segev, G. Raitses, J. M. Paratte
Nuclear Science and Engineering | Volume 131 | Number 1 | January 1999 | Pages 123-131
Technical Paper | doi.org/10.13182/NSE99-A2023
Articles are hosted by Taylor and Francis Online.
The radial distribution of capture rate and effective cross section in fuel rods of radii R, forming a light water reactor (LWR) lattice, is derived with routine cell calculations. Any internal radial subrange (r1,r2) is treated through the assessment of absorption in the two corresponding annular absorbers (r1,R) and (r2,R). The lattice of the latter absorbers, whose pitch is exactly the original LWR lattice pitch, is equivalenced to a lattice of solid cylindrical rods. Thus, for example, to obtain a tenfold radial distribution, ten routine cell calculations are required.In determining the radius s of a cylinder equivalent to the annulus (r,R), the neutron escape from the annulus is first preserved by making the s rod have a circumference of 2R[1 - (0.5 - (1/)cos-1(r/R))G], where G is the "sticking" probability in the annulus for neutrons entering it from within. The radius s is then the result of making the solid rod and the annulus have the same average chord. In addition, a lattice is assigned to the s rods such that the original Dancoff factor is preserved. Finally, a Bell factor is determined for the s rod such that the actual grayness of the annulus (r,R) is preserved.A special program for transport-related probabilities is invoked in obtaining the sticking and Dancoff probabilities just described, as well as the Bell factor.Application of the theory was conducted with the ELCOS system BOXER cell code. Three benchmarks were considered. The first was the one suggested by Tellier et al. for a fuel pin of a typical pressurized water reactor cell. The second was almost identical to the first, except that the fuel was saturated with hydrogen to generate a flatter radial distribution than in the first benchmark. The third benchmark was based on detailed space-energy calculations for a boiling water reactor rod, performed in 1978.All three benchmark testings resulted in satisfactory comparisons. Hence, the present theory may provide a practical, routine way of obtaining the in-rod distribution of absorption and cross section, calling just for a repeated use of straightforward cell calculations.
