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Fusion Science and Technology
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Glass strategy: Hanford’s enhanced waste glass program
The mission of the Department of Energy’s Office of River Protection (ORP) is to complete the safe cleanup of waste resulting from decades of nuclear weapons development. One of the most technologically challenging responsibilities is the safe disposition of approximately 56 million gallons of radioactive waste historically stored in 177 tanks at the Hanford Site in Washington state.
ORP has a clear incentive to reduce the overall mission duration and cost. One pathway is to develop and deploy innovative technical solutions that can advance baseline flow sheets toward higher efficiency operations while reducing identified risks without compromising safety. Vitrification is the baseline process that will convert both high-level and low-level radioactive waste at Hanford into a stable glass waste form for long-term storage and disposal.
Although vitrification is a mature technology, there are key areas where technology can further reduce operational risks, advance baseline processes to maximize waste throughput, and provide the underpinning to enhance operational flexibility; all steps in reducing mission duration and cost.
A. N. Perevezentsev, A. C. Bell, B. M. Andreev, M. B. Rozenkevich, Yu. S. Pak, A. V. Ovcharov
Fusion Science and Technology | Volume 56 | Number 4 | November 2009 | Pages 1455-1461
Technical Paper | doi.org/10.13182/FST56-1455
Articles are hosted by Taylor and Francis Online.
This paper evaluates detritiation of air contaminated with tritium in the form of water vapor using a scrubber column filled with structured packing. This technique is based on isotopic exchange between tritiated water vapor and liquid water. In combination with a catalytic oxidizer operated at room or slightly elevated temperature, the scrubber column can also decontaminate air contaminated with tritiated molecular hydrogen. Mass transfer rates measured for structured packings made of stainless steel and copper alloy confirmed high efficiency of the detritiation process. Study of the effect of various operation parameters on column efficiency allows optimization of column operation. It was demonstrated that this technique is competitive with the drying technique with respect to the decontamination factor (DF) provided and the amount of tritiated water to be generated. Benefits offered by the wet scrubber technology are based on the nature of the isotopic exchange process. No need for regeneration allows reduction in the number of units and as such decreases the capital cost of the facility for continuous operation. The DF can be controlled by changing the flow rate of feedwater.